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2020 | OriginalPaper | Buchkapitel

6. Chemical Speciation and Source Apportionment of Airborne Coarse Particles at Kanpur

verfasst von : Pragati Rai, Tarun Gupta

Erschienen in: Measurement, Analysis and Remediation of Environmental Pollutants

Verlag: Springer Singapore

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Abstract

The key objective of this study was to unravel the major sources of PM_10-2.5 (defined as PM₁₀-PM_2.5 or coarse particles) within and near the city of Kanpur. Airborne particulate matter (PM) samples were collected from 1st April to 15th July, 2011. The average mass concentration of coarse particles was found to be 64.3 ± 51.16 µg/m³. In addition to the mass concentrations of coarse particles their black carbon (BC), water soluble inorganic carbon (WSIC), water soluble organic carbon (WSOC), water-soluble ions and elemental composition were also determined. The size-resolved data set was processed via Positive Matrix Factorization (PMF) to carefully identify major sources and an attempt was made to quantify their respective source strengths. The contribution of these sources to the coarse PM mass concentration was also assessed. The identified sources and their contributions for the coarse particles were paved road dust (53%), vehicular emission (7%), coal combustion & brick kilns (2.5%), construction activities and incineration (0.5%), crustal dust (32%) and biomass burning and oil combustion (5%).

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Vorheriges Kapitel Organic Air Pollutants: Measurement, Properties & Control

Nächstes Kapitel Analysis of an Aerosol Environment in an Urban Region and Its Impact on Regional Meteorology

Amato F, Schaap M, Denier van der Gon HAC, Pandolfi M, Alastuey A, Keuken M, Querol X (2013) Short-term variability of mineral dust, metals and carbon emission from road dust resuspension. Atmos Environ 74:134–140CrossRef

Cesari DA, Ielpo GP, Siciliano M, Mascolo G, Grasso FM, Contini D (2014) Source apportionment of PM_2.5 in the harbour–industrial area of Brindisi (Italy): identification and estimation of the contribution of in-port ship emissions. Sci Total Environ 497–498:392–400CrossRef

Chakraborty A, Gupta T (2010) Chemical characterization and source apportionment of submicron (PM₁) aerosol in Kanpur Region. India Aeros Air Qual Res 10(5):433–445CrossRef

Chan YC, Hawas O, Hawker D, Vowles P, Cohen DD, Stelcer E, Simpson R, Golding G, Christensen E (2011) Using multiple type composition data and wind data in PMF analysis to apportion and locate sources of air pollutants. Atmos Environ 45:439–449CrossRef

Cheng Y, Lee S, Gu Z, Ho K, Zhanga Y, Huang Y, Chow JC, Watson JG, Cao J, Zhang R (2014) PM_2.5 and PM_10–2.5 chemical composition and source apportionment near a Hong Kong roadway. Particuology 30

Chinnam N, Dey S, Tripathi SN, Sharma M (2006) Dust events in Kanpur, northern India: chemical evidence for source and implications to radiative forcing. Geophys Res Lett 33:L08803CrossRef

Councell TB, Duckenfield KU, Landa ER, Callender E (2004) Tire-wear particles as a source of zinc to the environment. Environ Sci & Technol 38:4206–4214

Dey S, Tripathi SN, Singh RP, Holben BN (2004) Influence of dust storms on the aerosol optical properties over the Indo-Gangetic basin. J Geophys Res Atmos 109:20211CrossRef

Ethirajan R, Mohan S (2012) Comparative evaluation of VOC source profiles developed by PMF and UNMIX models. Int J Environ Sci Dev 3(5)

Ghosh S, Gupta T, Rastogi N, Gaur A, Misra A, Tripathi SN, Paul D, Tare V, Prakash O, Bhattu D, Dwivedi AK, Kaul DS, Dalai R, Mishra SK (2014) Chemical characterization of summertime dust events at Kanpur: insight into the sources and level of mixing with anthropogenic emissions. Aerosol Air Qual Res 14:879–891CrossRef

Gu JW, Pitz M, Schnelle–Kreis J, Diemer J, Reller A, Zimmermann R, Soentgen J, Toelzel M, Wichmann HE, Peters A, Cyrys J (2011) Source apportionment of ambient particles: comparison of positive matrix factorization analysis applied to particle size distribution and chemical composition data. Atmos Environ 45:1849–1857CrossRef

Gupta T, Mandariya A (2013) Sources of submicron aerosol during fog-dominated wintertime at Kanpur. Environ Sci Poll Res 20:5615–5629CrossRef

Hammond DM, Dvonch JT, Keeler GJ, Parker EA, Kamal AS, Barres JA, Yip FY, Brakefield-Caldwell W (2008) Sources of ambient fine particulate matter at two community sites in Detroit, Michigan. Atmos Environ 42:720–732CrossRef

Harrison RM, Smith DIT, Luhana L (1996) Source apportionment of atmospheric polycyclic aromatic hydrocarbons collected from an urban location in Birmingham, U.K. Environ Sci Tech 30(3):825–832CrossRef

Harrison RM, Shi JP, Xi SH, Khan A, Mark D, Kinnersley R (2000) Measurement of number, mass and size distribution of particles in the atmosphere. Philos Trans R Soc Lond Ser A 358:2567–2580CrossRef

Kulshrestha A, Satsangi PG, Masih J, Taneja A (2009) Metal concentration of PM_2.5 and PM₁₀ particles and seasonal variations in urban and rural environment of Agra, India. Sci Total Environ 407:6196–6204CrossRef

Kumar A, Srivastava D, Agrawal M, Goel A (2014) Snapshot of PM loads evaluated at major road and railway intersections in an urban locality. Int J Environ Prot 4(1):23–29

Kupiainen KJ, Tervahattu H, Raisanen M, Makela T, Aurela M, Hillamo R (2005) Size and composition of airborne particles from pavement wear, tires, and traction sanding. Environ Sci Technol 39:699–706CrossRef

Li R, Wiedinmyer C, Hannigan MP (2013) Contrast and correlations between coarse and fine particulate matter in the United States. Sci Total Environ 456–457:346–358CrossRef

Misra A, Gaur A, Bhattu D, Ghosh S, Dwivedi A, Dalai R, Paul D, Gupta T, Tare V, Singh S, Eck T, Welton E, Holben B, Tripathi SN, Mishra SK (2014) An overview of the physico-chemical characteristics of dust at Kanpur in the central Indo-Gangetic basin. Atmos Environ 97:386–396CrossRef

Nastos T, Athanasios G, Michael B, Eleftheria SR, Kostas NP (2010) Outdoor particulate matter and childhood asthma admission in Athens, Greece: a time-series study. Environ Health 9:1–9CrossRef

Norris GA, Duvall R, Brown SG, Bai S (2014) EPA positive matrix factorization (PMF) 5.0 fundamentals and user Guide prepared for the U.S. environmental protection agency office of research and development. Washington, DC. (EPA/600/R-14/108; STI-910511–5594-UG, April)

Owoade KO, Hopke PK, Olise FS, Ogundele LT, Fawole OG, Olaniyi BH, Jegede OO, Ayoola MA, Bashiru MI (2015) Chemical compositions and source identification of particulate matter (PM_2.5 and PM_2.5-10) from a scrap iron and steel smelting industry along the Ife-Ibadan highway. Nigeria Atmos Pollut Res 6:107–119CrossRef

Paatero P, Tapper U (1994) Positive matrix factorization: a non-negative factor model with optimal utilization of error estimates of data values. Environmetrics 5:111–126CrossRef

Paatero P, Eberly S, Brown SG, Norris GA (2014) Methods for estimating uncertainty in factor analytic solutions. Atmos Meas Tech 7:781–797CrossRef

Polissar AV, Hopke PK, Paatero P (1998) Atmospheric aerosol over Alaska-2. Elemental composition and sources. J Geophys Res-Atmos 103:19045–19057CrossRef

Querol X, Alastuey A, Moreno T, Viana MM, Castillo S, Pey J, Rodriguez S, Artinano B, Salvador P, Sanchez M, Garcia Dos Santos S, HerceGarraleta MD, Fernandez-Patier R, Moreno-Grau S, Negral L, Minguillon MC, Monfort E, Sanz MJ, Palomo-Marin R, Pinilla-Gil E, Cuevas E, de la Rosa J, Sanchez de la Campa A (2008) Spatial and temporal variations in airborne particulate matter (PM₁₀ and PM_2.5) across Spain 1999–2005. Atmos Environ 42:3964–3979CrossRef

Rajput P, Mandaria A, Kachawa L, Singh DK, Singh AK, Gupta T (2016) Chemical characterisation and source apportionment of PM₁ during massive loading at an urban location in Indo-Gangetic Plain: impact of local sources and long-range transport. Tellus B 68:30659CrossRef

Rajput P, Singh DK, Singh AK, Gupta T (2018) Chemical composition and source-apportionment of sub-micron particles during wintertime over Northern India: new insights on influence of fog-processing. Environ Pollut 233:81–91CrossRef

Rajput P, Izhar S, Gupta T (2019) Deposition modeling of ambient aerosols in human respiratory system: health implication of fine particles penetration into pulmonary region. Atmos Pollut Res 10:334–343CrossRef

Ram K, Sarin MM (2012) Carbonaceous aerosols over Northern India: sources and spatio-temporal variability. Proc Indian natnSciAcad 78(3):523–533

Rastogi N, Sarin MM (2009) Quantitative chemical composition and characteristics of aerosols over western India: one-year record of temporal variability. Atmos Environ 43:3481–3488CrossRef

Schleicher NJ, Norra S, Chai F, Chen Y, Wang S, Cen K, Yu Y, Stueben D (2011) Temporal variability of trace metal mobility of urban particulate matter from Beijing—A contribution to health impact assessments of aerosols. Atmos Environ 45:7248–7265CrossRef

Sharma SK, Mandal TK, Saxena M, Rashmi Sharma A, Datta A, Saud T (2014). Variation of OC, EC, WSIC and trace metals of PM₁₀ in Delhi, India. J Atmos Sol-Terr Phys 113:10–22CrossRef

Soluri DS, Godoy MLDP, Godoy JM, Roldão LA (2007). Multi-site PM_2.5 and PM_2.5–10 aerosol source apportionment in Rio de Janeiro, Brazil. J Braz Chem Soc 18(4):838–845CrossRef

Tao J, Zhang L, Engling G, Zhang R, Yang Y, Cao J, Zhu C, Wang Q, Luo L (2013) Chemical composition of PM_2.5 in an urban environment in Chengdu, China: importance of springtime dust storms and biomass burning. Atmos Res 122:270–283CrossRef

Uberol M, Shadman F (1991) High–temperature removal of cadmium compounds using solid sorbents. Environ Sci Technol 25:1285–1289CrossRef

Vedal S, Hannigan MP, Dutton SJ, Miller SL, Milford JB, Rabinovitch N, Kim SY, Sheppard L (2009) The denver aerosol sources and health (DASH) study: overview and early findings. Atmos Environ 43:1666–1673CrossRef

Vincent K, Passant N (2006) Assessment of heavy metal concentrations in the United Kingdom, AEA technology, http://uk-air.defra.gov.uk/assets/documents/reports/cat16/0604041205_heavy_metal_issue1_final.pdf

Visser S, Slowik JG, Furger M, Zotter P, Bukowiecki N, Canonaco F, Flechsig U, Appel K, Green DC, Tremper AH, Young DE, Williams PI, Allan JD, Coe H, Williams LR, Mohr C, Xu L, Ng NL, Nemitz E, Barlow JF, Halios CH, Fleming ZL, Baltensperger U, Prévôt ASH (2015) Advanced source apportionment of size-resolved trace elements at multiple sites in London during winter. Atmos Chem Phys 15:11291–11309CrossRef

Watson JG (2004) Desert research institute, protocol for applying and validating the CMB Model for PM_2.5 and VOC, US environmental protection agency, air quality modeling group

WHO (2013) Review of evidence on health aspects of air pollution–REVIHAAP Project, Report, WHO European Centre for Environment and Health, Bonn

Yang L, Cheng S, Wang X, Nie W, Xu P, Gao X, Yuan C, Wang W (2013) Source identification and health impact of PM_2.5 in a heavily polluted urban atmosphere in China. Atmos Environ 75:265–269CrossRef

Yang H, Chen J, Wen J, Tian H, Liu X (2015) Composition and sources of PM_2.5 around the heating periods of 2013 and 2014 in Beijing: implications for efficient mitigation measures. Atmos Environ 30:1–9

Yuan H, Zhuang G, Li J, Wang Z (2008) Mixing of mineral with pollution aerosols in dust season in beijing: revealed by source apportionment study. Atmos Environ 42:2141–2157CrossRef

Zhang R, Jing J, Tao J, Hsu S-C, Wang G, Cao J, Lee CSL, Zhu L, Chen Z, Zhao Y, Shen Z (2013) Chemical characterization and source apportionment of PM_2.5 in Beijing: seasonal perspective. Atmos Chem Phys 13:7053–7074CrossRef

Titel: Chemical Speciation and Source Apportionment of Airborne Coarse Particles at Kanpur
verfasst von: Pragati Rai
Tarun Gupta
Verlag: Springer Singapore
Buch: Measurement, Analysis and Remediation of Environmental Pollutants
Print ISBN: 978-981-15-0539-3

Electronic ISBN: 978-981-15-0540-9

Copyright-Jahr: 2020
DOI: https://doi.org/10.1007/978-981-15-0540-9_6