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Journal of Materials Science
Erschienen in: Journal of Materials Science 29/2020

17.07.2020 | Composites & nanocomposites

Construction of the rapid spatial charge migration core/shell heterostructure by ZnIn2S4 nanosheet-surface-loaded β-Bi2O3 for improved photooxidative performance

verfasst von: Yan Xiao, Yinhua Jiang, Xiaolong Liu, Wenli Zhang, Zhi Zhu, Yuhang Gao, Haiqing Xu, Jianming Zhang, Zhanchao Liu, Liang Ni

Erschienen in: Journal of Materials Science | Ausgabe 29/2020

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Abstract

The development of novel heterojunctions with optimized interface contact is essential for realizing the highly efficient solar conversion in photocatalysis. In this work, a series of β-Bi2O3/ZnIn2S4 (BO/ZIS) nanocomposite photocatalysts were firstly fabricated via a facile self-assembly process, in which a large number of ZnIn2S4 nanosheets were tightly loaded on β-Bi2O3 nanoparticles to form the unique core/shell heterostructure. The produced core/shell BO/ZIS hybrid heterojunction with larger contact areas could provide more high-speed charge transmission nanochannels for better spatial charge separation. The boosted charge carrier migration, extended spectral adsorption and increased surface areas were favorable for the enhancement of efficiency, thus contributing to the significantly improved tetracycline hydrochloride (TCH) photodegradation performance. In particular, the experimental results showed that the as-synthesized BO/ZIS-2 hybrid possessed the optimal degradation efficiency and its rate constant was about 1.84 and 2.49 times higher than those of bare β-Bi2O3 and Znln2S4, respectively. Furthermore, in accordance with the trapping analysis and HPLC–MS results, the predominant active specie acted during the reaction process and the degradation intermediate products of TCH were proposed. Finally, the possible reaction mechanism was put forward. This study verified that the construction of β-Bi2O3-based core/shell heterostructure was an effective strategy to improve its photocatalytic performance for its practical application.
Vorheriger Artikel Graphene-based intumescent flame retardant on cotton fabric
Nächster Artikel Synthesis and characterization of polymeric films with stress-altered aluminum particle fillers

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Metadaten
Titel
Construction of the rapid spatial charge migration core/shell heterostructure by ZnIn2S4 nanosheet-surface-loaded β-Bi2O3 for improved photooxidative performance
verfasst von
Yan Xiao
Yinhua Jiang
Xiaolong Liu
Wenli Zhang
Zhi Zhu
Yuhang Gao
Haiqing Xu
Jianming Zhang
Zhanchao Liu
Liang Ni
Publikationsdatum
17.07.2020
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 29/2020
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-020-05004-8

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