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Journal of Sol-Gel Science and Technology

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23.04.2022 | Invited Paper: Sol-gel and hybrid materials for optical, photonic and optoelectronic applications

Ammonia-free synthesis and color tuning of oxynitride perovskite SrTaO₂N-SrTiO₃ solid solution by using alkoxide-derived Ta-Ti binary oxide gel precursors

verfasst von: Takuya Sakata, Risa Yoshiyuki, Sohta Urushidani, Naoki Tarutani, Kiyofumi Katagiri, Kei Inumaru

Erschienen in: Journal of Sol-Gel Science and Technology | Ausgabe 3/2022

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Abstract

Solid solutions of strontium-tantalum oxynitride perovskite (SrTaO₂N) and strontium-titanium oxide perovskite (SrTiO₃) were prepared as possible candidates for novel inorganic pigments. The use of Ta-Ti binary oxide gel, which was obtained by the sol–gel method, was conducive to the development of single-phase solid solutions with a homogeneous atomic distribution. In addition, the use of urea as a nitriding agent availed to eliminate harmful ammonia gas during the synthesis. The color of solid solution depends on the band gap and Ti reduction state, which changes with Ti content. As a result, various chromatic colors, i.e., orange to yellow-green, were obtained from solid solutions. The solid solutions retained their color even after thermal and chemical resistance examinations. Because toxic substances were eliminated from the products and preparation process, the solid solutions show potentials to be applied as environmentally-friendly pigments.

Vorheriger Artikel Fundamental properties of alkoxide-derived titania gel films providing plastics surface with high refractive index

Nächster Artikel Redox-induced dual optical switching of CaTiO3:Pr3+ phosphor nanoparticles synthesized by sol–gel method

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Titel: Ammonia-free synthesis and color tuning of oxynitride perovskite SrTaO2N-SrTiO3 solid solution by using alkoxide-derived Ta-Ti binary oxide gel precursors
verfasst von: Takuya Sakata
Risa Yoshiyuki
Sohta Urushidani
Naoki Tarutani
Kiyofumi Katagiri
Kei Inumaru
Publikationsdatum: 23.04.2022
Verlag: Springer US
Erschienen in: Journal of Sol-Gel Science and Technology / Ausgabe 3/2022
Print ISSN: 0928-0707
Elektronische ISSN: 1573-4846
DOI: https://doi.org/10.1007/s10971-022-05801-4

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