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2019 | OriginalPaper | Buchkapitel

1. An Historical Perspective on Fission-Track Thermochronology

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Abstract

This chapter reviews the background, beginnings and early development of fission-track (FT) thermochronology. In the 1930s, it was discovered that uranium would break into two lighter products when bombarded with neutrons and, subsequently, that uranium was capable of natural, spontaneous fission. The fission process produced damage tracks in solid-state detectors, which could be revealed by chemical etching and observed by electron and, later, by optical microscopy. Fleischer, Price and Walker at the General Electric R&D laboratories developed diverse track-etching procedures, estimates of track registration and stability in different materials, track formation models, uranium determination in terrestrial, lunar and meteorite samples, neutron dosimetry and mineral dating using 238U spontaneous fission. Application to dating of natural and man-made glass was frustrated by low-uranium content and relative ease of track fading (annealing). In the 1970s–1980s, most FT analyses used apatite, zircon and titanite (sphene) to date tephra and acid intrusive rocks with the recognition of differing sensitivities of track annealing in each mineral. Studies in the Alps showed apatite with its greater susceptibility to annealing could provide estimates of the timing and rate of exhumation. The landmark 1980 Pisa FT Workshop highlighted problems with FT system calibration and emphasised the value of annealing in apatite to reveal thermal history. System calibration eventually reached a consensus agreement in 1988 at the Besançon FT Workshop with the majority of analysts adopting the zeta comparative approach. Multiple laboratory and borehole studies have determined the conditions for track annealing in apatite leading to widespread applications in exhumation, sedimentary basin, hydrocarbon exploration and other areas.

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Fußnoten
1
Spontaneous fission also occurs in 234U, 235U and 232Th, but their spontaneous fission half-lives are too long and/or abundances too low to produce significant numbers of natural tracks compared to 238U.
 
2
4th International Conference on Geochronology, Cosmochronology and Isotope Geology (ICOG) in August 1978 at Snowmass-at-Aspen, Colorado, USA.
 
3
Note the Pisa workshop is sometimes regarded as the first FT Dating Workshop and is so titled in the Proceedings. However, strictly it was the second such workshop, the first being within the 4th ICOG in 1978, which initiated the Pisa Workshop. Subsequent FT Workshops have followed this latter numbering convention.
 
4
Neutron irradiation induces fission in a proportion of 235U in a sample as a measure of its uranium content and requires determination of the total number of neutrons to which the sample is exposed, known as the neutron fluence. Fluence is the neutron flux (or dose) integrated with respect to the irradiation time and is expressed in neutrons cm−2.
 
5
Cadmium absorbs thermal neutrons (<~0.4 eV) whilst permitting higher energy neutrons passage through. A cadmium ratio gives the activities of a bare monitor/ a Cd-shielded monitor, thus recording neutrons of all energies/neutrons with energies >0.5 eV; the higher the cadmium ratio, the better thermalised the reactor facility.
 
6
Hydrostatic pressure, static shear stress, fluids, irradiation with non-track forming particles and weathering appear to have no, or minimal affect on annealing of tracks in crystalline materials although may cause some modification in glasses. Chemical composition may have significant changes in track annealing rates, in particular variation of the F/Cl ratios of apatite—see Chap. 3, Ketcham 2018.
 
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Metadaten
Titel
An Historical Perspective on Fission-Track Thermochronology
verfasst von
Anthony J. Hurford
Copyright-Jahr
2019
DOI
https://doi.org/10.1007/978-3-319-89421-8_1