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Journal of Materials Engineering and Performance

Erschienen in:

30.01.2020

Confinement of Mg Nanoparticles by Bituminous Coal and Associated Synergistic Hydrogen Storage Effect

verfasst von: Yanwei Song, Tonghuan Zhang, Shixue Zhou, Pei Liu, Hao Yu, Zongying Han

Erschienen in: Journal of Materials Engineering and Performance | Ausgabe 2/2020

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Abstract

Using the coking property of bituminous coal, a nanostructured Mg-C composite hydrogen storage material was developed by ball milling and heat treatment. The heat treatment conditions and hydrogen storage behavior of the composite material were investigated. Results show that when the material is heat-treated at 550 °C under Ar atmosphere, the carbon could react with Mg to irreversibly form Mg₂C₃. When 1.0 MPa H₂ was introduced to the heat treatment at 550 °C, the magnesium does not form Mg₂C₃. The resulting composite material is shown to have a globular bonded structure by scanning electron microscopy, and the Mg nanoparticles are confined by the bituminous coal. Fourier transform infrared spectroscopy and gas chromatography analysis show that the carbon could combine with hydrogen only in the presence of MgH₂ under current experimental conditions. The carbon-bonded hydrogen would be released in the form of small molecule hydrocarbons such as CH₄, C₂H₄ and C₂H₆. Dynamic tests show that coal carbon and magnesium absorb/desorb hydrogen at similar temperatures, which proves that there is a synergistic hydrogen storage effect between magnesium and coal carbon.

Vorheriger Artikel Experimental Investigation on Friction-Stir-Assisted Incremental Forming with Synchronous Bonding of Aluminum Alloy and Steel Sheets

Nächster Artikel Quantitative Analysis of Strengthening Effect Contributed by Microstructure Characteristics in Pure Titanium Consolidated by Severe Plastic Deformation

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Titel: Confinement of Mg Nanoparticles by Bituminous Coal and Associated Synergistic Hydrogen Storage Effect
verfasst von: Yanwei Song
Tonghuan Zhang
Shixue Zhou
Pei Liu
Hao Yu
Zongying Han
Publikationsdatum: 30.01.2020
Verlag: Springer US
Erschienen in: Journal of Materials Engineering and Performance / Ausgabe 2/2020
Print ISSN: 1059-9495
Elektronische ISSN: 1544-1024
DOI: https://doi.org/10.1007/s11665-020-04602-6

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