nach oben

Journal of Materials Science

Erschienen in:

30.11.2020 | Chemical routes to materials

Cu/MgO and Ni/MgO composite nanoparticles for fast, high-efficiency adsorption of aqueous lead(II) and chromium(III) ions

verfasst von: Iryna Matsukevich, Yuliya Lipai, Valentin Romanovski

Erschienen in: Journal of Materials Science | Ausgabe 8/2021

Einloggen

Aktivieren Sie unsere intelligente Suche, um passende Fachinhalte oder Patente zu finden.

search-config

KI-gestützte Suche

Aus

Abstract

The conditions were found and the patterns of formation of Ni and Cu composites based on MgO, obtained by the precipitation method and by the glycine–citrate–nitrate method. The obtained materials are of interest as sorbents for the purification of aqueous media from toxic impurities, as well as catalysts in organic synthesis, in particular for the production of methanol from carbon dioxide. The phase composition, thermal stability, microstructure of obtained nanocomposites, as well as their sorption properties, were studied. It was found that high sorption capacities of powders of magnesium oxide and MgO-M (where M—Cu, Ni) nanocomposites with respect to lead and chromium ions are up to 2989.0 and 499.9 mg/g, respectively.

Vorheriger Artikel Separable magnetic MoS2@Fe3O4 nanocomposites with multi-exposed active edge facets toward enhanced adsorption and catalytic activities

Nächster Artikel The nano-composite of Co-doped g-C3N4 and ZnO sensors for the rapid detection of BTEX gases: stability studies and gas sensing mechanism

Sie haben noch keine Lizenz? Dann Informieren Sie sich jetzt über unsere Produkte:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

über 102.000 Bücher
über 537 Zeitschriften

aus folgenden Fachgebieten:

Automobil + Motoren
Bauwesen + Immobilien
Business IT + Informatik
Elektrotechnik + Elektronik
Energie + Nachhaltigkeit
Finance + Banking
Management + Führung
Marketing + Vertrieb
Maschinenbau + Werkstoffe
Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

Jetzt informieren

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

über 67.000 Bücher
über 390 Zeitschriften

aus folgenden Fachgebieten:

Automobil + Motoren
Bauwesen + Immobilien
Business IT + Informatik
Elektrotechnik + Elektronik
Energie + Nachhaltigkeit
Maschinenbau + Werkstoffe

Jetzt Wissensvorsprung sichern!

Jetzt informieren

Krasae N, Wantala K (2016) Enhanced nitrogen selectivity for nitrate reduction on Cu–nZVI by TiO2 photocatalysts under UV irradiation. Appl Surf Sci 380:309–317. https://doi.org/10.1016/j.apsusc.2015.12.023CrossRef

Wang C, Luo H, Zhang Z, Wu Y, Zhang J, Chen S (2014) Removal of As (III) and As (V) from aqueous solutions using nanoscale zero valent iron-reduced graphite oxide modified composites. J Hazard Mater 268:124–131. https://doi.org/10.1016/j.jhazmat.2014.01.009CrossRef

Zhou Q, Lei M, Li J, Zhao K, Liu Y (2017) Sensitive determination of bisphenol A, 4-nonylphenol and 4-octylphenol by magnetic solid phase extraction with Fe@MgAl-LDH magnetic nanoparticles from environmental water samples. Sep Purif Technol 182:78–86. https://doi.org/10.1016/j.seppur.2017.01.071CrossRef

Liu M, Wang Y, Chen L, Zhang Y, Lin Z (2015) Mg(OH)2 supported nanoscale zero valent iron enhancing the removal of Pb(II) from aqueous solution. ACS Appl Mater Interfaces 7(15):7961–7969. https://doi.org/10.1021/am509184eCrossRef

Liu W, Ma J, Sun S, Chen K (2016) Gram-grade Cr (VI) adsorption on porous Fe@SiO2 hierarchical microcapsules. J Water Process Eng 12:111–119. https://doi.org/10.1016/j.jwpe.2016.07.003CrossRef

Weng X, Cai W, Lin S, Chen Z (2017) Degradation mechanism of amoxicillin using clay supported nanoscale zero-valent iron. Appl Clay Sci 147:137–142. https://doi.org/10.1016/j.clay.2017.07.023CrossRef

Peng Q, Dai Y, Liu K, Luo X, He D, Tang X, Huang G (2020) A novel carbon nanotube–magnesium oxide composite with excellent recyclability to efficiently activate peroxymonosulfate for Rhodamine B degradation. J Mater Sci 55:11267–11283. https://doi.org/10.1007/s10853-020-04822-0CrossRef

Khort A, Romanovski V, Leybo D, Moskovskikh D (2020) CO oxidation and organic dyes degradation over graphene-Cu and graphene-CuNi catalysts obtained by solution combustion synthesis. Sci Rep 10:16104. https://doi.org/10.1038/s41598-020-72872-0CrossRef

Huang J, Li X, Wang X, Fang X, Wang H, Xu X (2019) New insights into CO2 methanation mechanisms on Ni/MgO catalysts by DFT calculations: elucidating Ni and MgO roles and support effects. J CO2 Util 33:55–63. https://doi.org/10.1016/j.jcou.2019.04.022CrossRef

10.

Charisiou ND, Papageridis KN, Tzounis L, Sebastian V, Hinder SJ, Baker MA, AlKetbi M, Polychronopoulou K, Goula MA (2019) Ni supported on CaO-MgO-Al2O3 as a highly selective and stable catalyst for H2 production via the glycerol steam reforming reaction. Int J Hydrog Energy 44(1):256–273. https://doi.org/10.1016/j.ijhydene.2018.02.165CrossRef

11.

Li J, Li J, Zhu Q, Li H (2018) Magnetic field acceleration of CO2 reforming of methane over novel hierarchical Co/MgO catalyst in fluidized bed reactor. Chem Eng J 350:496–506. https://doi.org/10.1016/j.cej.2018.05.034CrossRef

12.

Feng X, Feng J, Li W (2018) Insight into MgO promoter with low concentration for the carbon-deposition resistance of Ni-based catalysts in the CO2 reforming of CH4. Chin J Catal 39(1):88–98. https://doi.org/10.1016/S1872-2067(17)62928-0CrossRef

13.

Li X, Huang Y, Zhang Q, Luan C, Vinokurov VA, Huang W (2019) Highly stable and anti-coking Ni/MoCeZr/MgAl2O4-MgO complex support catalysts for CO2 reforming of CH4: effect of the calcination temperature. Energy Convers Manag 179:166–177. https://doi.org/10.1016/j.enconman.2018.10.067CrossRef

14.

Dasireddy VD, Neja SŠ, Blaž L (2018) Correlation between synthesis pH, structure and Cu/MgO/Al2O3 heterogeneous catalyst activity and selectivity in CO2 hydrogenation to methanol. J CO2 Util 28:189–199. https://doi.org/10.1016/j.jcou.2018.09.002CrossRef

15.

Ge L, Wang W, Peng Z, Tan F, Wang X, Chen J, Qiao X (2018a) Facile fabrication of Fe@ MgO magnetic nanocomposites for efficient removal of heavy metal ion and dye from water. Powder Technol 326:393–401. https://doi.org/10.1016/j.powtec.2017.12.003CrossRef

16.

Fajardo C, Gil-Díaz M, Costa G, Alonso J, Guerrero AM, Nande M, Lobo MC, Martín M (2015) Residual impact of aged nZVI on heavy metal-polluted soils. Sci Total Environ 535:79–84. https://doi.org/10.1016/j.scitotenv.2015.03.067CrossRef

17.

Su C, Puls RW (2004) Nitrate reduction by zerovalent iron: effects of formate, oxalate, citrate, chloride, sulfate, borate, and phosphate. Environ Sci Technol 38(9):2715–2720. https://doi.org/10.1021/es034650pCrossRef

18.

Dargahi A, Golestanifar H, Darvishi P, Karam A (2015) An investigation and comparison of removing heavy metals (lead and chromium) from aqueous solutions using magnesium oxide nanoparticles. Pol J Environ Stud 25:557–562. https://doi.org/10.15244/pjoes/60281CrossRef

19.

Tian G, Wang W, Zong L, Wang A (2017) MgO/palygorskite adsorbent derived from natural Mg-rich brine and palygorskite for high-efficient removal of Cd (II) and Zn (II) ions. J Environ Chem Eng 5(1):1027–1036. https://doi.org/10.1016/j.jece.2017.01.028CrossRef

20.

Ciesielczyk F, Bartczak P, Jesionowski T (2016) Removal of cadmium (II) and lead (II) ions from model aqueous solutions using sol–gel-derived inorganic oxide adsorbent. Adsorption 22(4–6):445–458. https://doi.org/10.1007/s10450-015-9703-7CrossRef

21.

Feng J, Gao M, Zhang Z, Liu S, Zhao X, Ren Y, Lv Y, Fan Z (2018) Fabrication of mesoporous magnesium oxide nanosheets using magnesium powder and their excellent adsorption of Ni (II). J colloid Interface Sci 510:69–76. https://doi.org/10.1016/j.jcis.2017.09.047CrossRef

22.

Matsukevich IV, Krutko NP, Ovseenko LV, Polhovskaja OV, Hubitski DV, Vashook VV (2018) Effect of preparation method on physicochemical properties of nanostructured MgO powder. Proc Natl Acad Sci Belarus Chem Ser 54(3):281–288. https://doi.org/10.29235/1561-8331-2018-54-3-281-288CrossRef

23.

Thommes M, Kaneko K, Neimark AV, Olivier JP, Rodriguez-Reinoso F, Rouquerol J, Sing KS (2015) Physisorption of gases, with special reference to the evaluation of surface area and pore size distribution (IUPAC Technical Report). Pure Appl Chem 87(9–10):1051–1069. https://doi.org/10.1515/pac-2014-1117CrossRef

24.

Li X, Xiao W, He G, Zheng W, Yu N, Tan M (2012) Pore size and surface area control of MgO nanostructures using a surfactant-templated hydrothermal process: high adsorption capability to azo dyes. Colloids Surf A Physicochem Eng Asp 408:79–86. https://doi.org/10.1016/j.colsurfa.2012.05.034CrossRef

25.

Matsukevich IV, Rucheys AN, Krutko NP, Kulbitskaia LV, Kuznetsova TF, Vashook VV (2017) Synthesis and adsorption properties of nanostructured powders Mg(OH)2 and MgO. Proc Nat Acad Sci Belarus Chem Ser 4:38–44

26.

Purwajanti S, Zhou L, Ahmad Nor Y, Zhang J, Zhang H, Huang X, Yu C (2015) Synthesis of magnesium oxide hierarchical microspheres: a dual-functional material for water remediation. ACS Appl Mater Interfaces 7(38):21278–21286. https://doi.org/10.1021/acsami.5b05553CrossRef

27.

Vedyagin AA, Mishakov IV, Karnaukhov TM, Krivoshapkina EF, Ilyina EV, Maksimova TA, Cherepanova SV, Krivoshapkin PV (2017) Sol–gel synthesis and characterization of two-component systems based on MgO. J Sol-Gel Sci Technol 82(2):611–619. https://doi.org/10.1007/s10971-017-4321-3CrossRef

28.

Xiong C, Wang W, Tan F, Luo F, Chen J, Qiao X (2015) Investigation on the efficiency and mechanism of Cd (II) and Pb (II) removal from aqueous solutions using MgO nanoparticles. J Hazard Mater 299:664–674. https://doi.org/10.1016/j.jhazmat.2015.08.008CrossRef

29.

Ngambia A, Ifthikar J, Shahib II, Jawad A, Shahzad A, Zhao M, Wang J, Chen Zh, Chen Z (2019) Adsorptive purification of heavy metal contaminated wastewater with sewage sludge derived carbon-supported Mg (II) composite. Sci Total Environ 691:306–321. https://doi.org/10.1016/j.scitotenv.2019.07.003CrossRef

30.

Zhang L, Zhu W, Zhang H, Bi S, Zhang Q (2014) Hydrothermal–thermal conversion synthesis of hierarchical porous MgO microrods as efficient adsorbents for lead (II) and chromium (VI) removal. RSC Adv 4(58):30542–30550. https://doi.org/10.1039/C4RA03971HCrossRef

31.

Cao CY, Qu J, Wei F, Liu H, Song WG (2012) Superb adsorption capacity and mechanism of flowerlike magnesium oxide nanostructures for lead and cadmium ions. ACS Appl Mater Interfaces 4(8):4283–4287. https://doi.org/10.1021/am300972zCrossRef

32.

Ge L, Wang W, Peng Z, Tan F, Wang X, Chen J, Qiao X (2018b) Facile fabrication of Fe@MgO magnetic nanocomposites for efficient removal of heavy metal ion and dye from water. Powder Technol 326:393–401. https://doi.org/10.1016/j.powtec.2017.12.003CrossRef

33.

Xu C, Yu Z, Yuan K, Jin X, Shi S, Wang X, Zhu L, Zhang G, Xu D, Jiang H (2019) Improved preparation of electrospun MgO ceramic fibers with mesoporous structure and the adsorption properties for lead and cadmium. Ceram Int 45(3):3743–3753CrossRef

34.

Chai Z, Tian Q, Ye J, Zhang S, Wang G, Qi Y, Che Y, Ning G (2020) Hierarchical magnesium oxide microspheres for removal of heavy ions from water and efficient bacterial inactivation. J Mater Sci 55(10):4408–4419. https://doi.org/10.1007/s10853-019-04312-yCrossRef

35.

Mahdavi S, Jalali M, Afkhami A (2013) Heavy metals removal from aqueous solutions using TiO2, MgO, and Al2O3 nanoparticles. Chem Eng Commun 200(3):448–470. https://doi.org/10.1080/00986445.2012.686939CrossRef

36.

Chen G, Shi L (2017) Removal of Cd (II) and Pb (II) ions from natural water using a low-cost synthetic mineral: behavior and mechanisms. RSC Adv 7(69):43445–43454. https://doi.org/10.1039/c7ra08018bCrossRef

37.

Pietrelli L, Francolini I, Piozzi A, Sighicelli M, Silvestro I, Vocciante M (2020) Chromium (III) removal from wastewater by chitosan flakes. Appl Sci 10(6):1925. https://doi.org/10.3390/app10061925CrossRef

38.

Keshavarz M, Foroutan R, Papari F, Bulgariu L, Esmaeili H (2020) Synthesis of CaO/Fe2O3 nanocomposite as an efficient nanoadsorbent for the treatment of wastewater containing Cr (III). Sep Sci Technol. https://doi.org/10.1080/01496395.2020.1778727

39.

Daniel AB, Zahir E, Hussain I, Naz S, Asghar MA (2020) Citric acid modified cellulose: a cost effective adsorbent for the immobilization of Cr (III) ions from the aqueous phase. Energy Sources Part A Recovery Util Environ Eff. https://doi.org/10.1080/15567036.2020.1773963

Titel: Cu/MgO and Ni/MgO composite nanoparticles for fast, high-efficiency adsorption of aqueous lead(II) and chromium(III) ions
verfasst von: Iryna Matsukevich
Yuliya Lipai
Valentin Romanovski
Publikationsdatum: 30.11.2020
Verlag: Springer US
Erschienen in: Journal of Materials Science / Ausgabe 8/2021
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI: https://doi.org/10.1007/s10853-020-05593-4

Premium Partner

Marktübersichten

Die im Laufe eines Jahres in der „adhäsion“ veröffentlichten Marktübersichten helfen Anwendern verschiedenster Branchen, sich einen gezielten Überblick über Lieferantenangebote zu verschaffen.

Zur Marktübersicht

Springer Professional

Abstract

Bitte loggen Sie sich ein, um Zugang zu Ihrer Lizenz zu erhalten.

Sie haben noch keine Lizenz? Dann Informieren Sie sich jetzt über unsere Produkte:

Springer Professional "Wirtschaft+Technik"

Springer Professional "Technik"

Weitere Artikel der Ausgabe 8/2021

Microstructure and tribomechanical properties of multilayer TiZrN/TiSiN composite coatings with nanoscale architecture by cathodic-arc evaporation

Friction stir welding of novel T-phase strengthened Zn-modified Al–Mg alloy

The mechanism of negative linear thermal expansion behavior of cold-rolled Ti-34Nb alloy

High impact resistance of a TWIP β titanium alloy: linking the multi-scale deformation and fracture mechanisms

The nano-composite of Co-doped g-C3N4 and ZnO sensors for the rapid detection of BTEX gases: stability studies and gas sensing mechanism

Gradient multilayer aluminium sheets used in automotive heat exchangers

Premium Partner

Marktübersichten