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Topics in Catalysis
Erschienen in: Topics in Catalysis 15-17/2013

01.11.2013 | Original Paper

D. W. (“Wayne”) Goodman: A Pioneer in Elucidating the Relationships Between Surface Structure of Catalysts and Their Performance, and in Using Model Catalysts for That Purpose

verfasst von: Charles T. Campbell

Erschienen in: Topics in Catalysis | Ausgabe 15-17/2013

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Excerpt

This special issue on “Structure/Function Relationships in Heterogeneous Catalysis: Insights using Well-Defined Model Catalysts” is dedicated to the memory of Professor D. Wayne Goodman for his many seminal contributions to our understanding of heterogeneous catalysis. His creative experiments using well-defined model catalysts decisively identified many surface structure–function relationships for bimetallic catalysts and oxide-supported metal nanoparticle catalysts and their underlying mechanistic explanations. Goodman is internationally recognized for his highly impactful contributions which truly paved the way for many of the other groups who later became active in this arena. His papers and talks in this area eloquently outlined how one could approach industrially-important fundamental questions in catalysis. Many researchers picked up on the excitement and clear-headed logic he projected in his talks, subsequently shifting their own research to use the new approaches he had established. As much as any other researcher, Prof. Goodman set the direction for the field of surface chemistry research related to heterogeneous catalysis from 1980 until 2010. …
Nächster Artikel Investigations of Structure Sensitivity in Heterogeneous Catalysis: From Single Crystals to Monodisperse Nanoparticles

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Literatur
1.
Goodman DW, Kelley RD, Madey TE, Yates JT (1980) Kinetics of the hydrogenation of CO over a single-crystal nickel-catalyst. J Catal 63:226–234CrossRef
2.
Goodman DW, White JM (1979) Measurement of active-carbon on ruthenium(110)—relevance to catalytic methanation. Surf Sci 90:201–203CrossRef
3.
Goodman DW, Kelley RD, Madey TE, White JM (1980) Measurement of carbide buildup and removal kinetics on Ni(100). J Catal 64:479–481CrossRef
4.
Goodman DW, Kiskinova M (1981) Chemisorption and reactivity studies of H2 and CO on sulfided Ni(100). Surf Sci 105:L265–L270CrossRef
5.
Kiskinova M, Goodman DW (1981) Modification of chemisorption properties by electronegative adatoms—H2 and CO on chlorided, sulfided, and phosphided Ni(100). Surf Sci 108:64–76CrossRef
6.
Kiskinova M, Goodman DW (1981) Interaction of H2 and CO with carbided and nitrided Ni(100). Surf Sci 109:L555–L559CrossRef
7.
Campbell CT, Goodman DW (1982) A surface science investigation of the role of potassium additives in nickel catalysts for CO hydrogenation. Surf Sci 123:413–426CrossRef
8.
Berlowitz PJ, Peden CHF, Goodman DW (1988) Kinetics of CO oxidation on single-crystal Pd, Pt and Ir. J Phys Chem 92:5213–5221CrossRef
9.
Goodman DW, Peden CHF (1986) CO oxidation over Rh and Ru—a comparative-study. J Phys Chem 90:4839–4843CrossRef
10.
Oh SH, Fisher GB, Carpenter JE, Goodman DW (1986) Comparative kinetic-studies of CO–O2 and CO–NO reactions over single-crystal and supported rhodium catalysts. J Catal 100:360–376CrossRef
11.
Peden CHF, Goodman DW (1986) Kinetics of CO oxidation over Ru(0001). J Phys Chem 90:1360–1365CrossRef
12.
Peden CHF, Goodman DW, Blair DS, Berlowitz PJ, Fisher GB, Oh SH (1988) Kinetics of CO oxidation by O2 or NO on Rh(111) and Rh(100) single-crystals. J Phys Chem 92:1563–1567CrossRef
13.
Beebe TP, Goodman DW, Kay BD, Yates JT (1987) Kinetics of the activated dissociative adsorption of methane on the low index planes of nickel single-crystal surfaces. J Chem Phys 87:2305–2315CrossRef
14.
Sault AG, Goodman DW (1988) Dissociative adsorption of alkanes on Ni(100)—comparison with molecular-beam results. J Chem Phys 88:7232–7239CrossRef
15.
Engstrom JR, Goodman DW, Weinberg WH (1986) Hydrogenolysis of n-butane over the (111) and (110)-(1×2) surfaces of iridium— a direct correlation between catalytic selectivity and surface-structure. J Am Chem Soc 108:4653–4655CrossRef
16.
Greenlief CM, Berlowitz PJ, Goodman DW, White JM (1987) CO methanation and ethane hydrogenolysis over Ni thin-films supported on w(110) and w(100). J Phys Chem 91:6669–6673CrossRef
17.
Peden CHF, Goodman DW (1987) Kinetics of cyclohexane dehydrogenation and hydrogenolysis over Ru(0001) and Cu/Ru(0001). J Catal 104:347–358CrossRef
18.
Rodriguez JA, Goodman DW (1991) Surface science studies of the electronic and chemical-properties of bimetallic systems. J Phys Chem 95:4196–4206CrossRef
19.
Rodriguez JA, Campbell RA, Goodman DW (1991) Electron-donor electron-acceptor interactions in bimetallic surfaces–theory and XPS studies. J Phys Chem 95:5716–5719CrossRef
20.
Rodriguez JA, Goodman DW (1992) The nature of the metal metal bond in bimetallic surfaces. Science 257:897–903CrossRef
21.
Chen MS, Kumar D, Yi CW, Goodman DW (2005) The promotional effect of gold in catalysis by palladium-gold. Science 310:291–293CrossRef
22.
Wu MC, Corneille JS, Estrada CA, He JW, Goodman DW (1991) Synthesis and characterization of ultra-thin MgO films on Mo(100). Chem Phys Lett 182:472–478CrossRef
23.
He JW, Estrada CA, Corneille JS, Wu MC, Goodman DW (1992) CO adsorption on ultrathin MgO films grown on a MO(100) surface—an iras study. Surf Sci 261:164–170CrossRef
24.
Wu MC, Truong CM, Goodman DW (1992) Electron-energy-loss-spectroscopy studies of thermally generated defects in pure and lithium-doped MgO(100) films on Mo(100). Phys Rev B 46:12688–12694CrossRef
25.
Wu MC, Corneille JS, He JW, Estrada CA, Goodman DW (1992) Preparation, characterization, and chemical-properties of ultrathin MgO films on MO(100). J Vac Sci Technol A 10:1467–1471CrossRef
26.
Xu XP, Goodman DW (1992) New approach to the preparation of ultrathin silicon dioxide films at low-temperatures. Appl Phys Lett 61:774–776CrossRef
27.
Xu XP, Vesecky SM, Goodman DW (1992) Infrared reflection-absorption spectroscopy and STM studies of model silica-supported copper-catalysts. Science 258:788–790CrossRef
28.
Xu XP, Goodman DW (1993) An infrared and kinetic-study of CO oxidation on model silica-supported palladium catalysts from 10−9 to 15-torr. J Phys Chem 97:7711–7718CrossRef
29.
Chen PJ, Goodman DW (1994) Epitaxial-growth of ultrathin Al2O3 films on Ta(110). Surf Sci 312:L767–L773CrossRef
30.
Xu XP, Chen PJ, Goodman DW (1994) A comparative-study of the coadsorption of CO and NO on Pd(100), Pd(111), and silica-supported palladium particles with infrared reflection-absorption spectroscopy. J Phys Chem 98:9242–9246CrossRef
31.
Rainer DR, Vesecky SM, Koranne M, Oh WS, Goodman DW (1997) The CO + NO reaction over Pd: a combined study using single-crystal, planar-model-supported, and high-surface-area Pd/Al2O3 catalysts. J Catal 167:234–241CrossRef
32.
Street SC, Xu C, Goodman DW (1997) The physical and chemical properties of ultrathin oxide films. Annu Rev Phys Chem 48:43–68CrossRef
33.
Rainer DR, Goodman DW (1998) Metal clusters on ultrathin oxide films: model catalysts for surface science studies. J Mol Catal A 131:259–283CrossRef
34.
Chusuei CC, Lai X, Luo K, Goodman DW (2001) Modeling heterogeneous catalysts: metal clusters on planar oxide supports. Top Catal 14:71–83CrossRef
35.
Goodman DW (1995) Model studies in catalysis using surface science probes. Chem Rev 95:523–536CrossRef
36.
Xu C, Lai X, Zajac GW, Goodman DW (1997) Scanning tunneling microscopy studies of the TiO2(110) surface: structure and the nucleation growth of Pd. Phys Rev B 56:13464–13482CrossRef
37.
Lai X, St Clair TP, Valden M, Goodman DW (1998) Scanning tunneling microscopy studies of metal clusters supported on TiO2 (110): morphology and electronic structure. Prog Surf Sci 59:25–52CrossRef
38.
Valden M, Lai X, Goodman DW (1998) Onset of catalytic activity of gold clusters on titania with the appearance of nonmetallic properties. Science 281:1647–1650CrossRef
39.
Valden M, Pak S, Lai X, Goodman DW (1998) Structure sensitivity of CO oxidation over model Au/TiO2 catalysts. Catal Lett 56:7–10CrossRef
40.
Lai XF, Goodman DW (2000) Structure-reactivity correlations for oxide-supported metal catalysts: new perspectives from STM. J Mol Catal A 162:33–50CrossRef
41.
Choudhary TV, Goodman DW (2002) Oxidation catalysis by supported gold nano-clusters. Top Catal 21:25–34CrossRef
42.
Goodman DW (2003) Model catalysts: from imagining to imaging a working surface. J Catal 216:213–222CrossRef
43.
Chen MS, Goodman DW (2004) The structure of catalytically active gold on titania. Science 306:252–255CrossRef
44.
Meier DC, Goodman DW (2004) The influence of metal cluster size on adsorption energies: CO adsorbed on Au clusters supported on TiO2. J Am Chem Soc 126:1892–1899CrossRef
45.
Chen MS, Goodman DW (2006) Catalytically active gold: From nanoparticles to ultrathin films. Acc Chem Res 39:739–746CrossRef
46.
Chen MS, Goodman DW (2006) Structure-activity relationships in supported Au catalysts. Catal Today 111:22–33CrossRef
47.
Chen MS, Goodman DW (2008) Catalytically active gold on ordered titania supports. Chem Soc Rev 37:1860–1870CrossRef
Metadaten
Titel
D. W. (“Wayne”) Goodman: A Pioneer in Elucidating the Relationships Between Surface Structure of Catalysts and Their Performance, and in Using Model Catalysts for That Purpose
verfasst von
Charles T. Campbell
Publikationsdatum
01.11.2013
Verlag
Springer US
Erschienen in
Topics in Catalysis / Ausgabe 15-17/2013
Print ISSN: 1022-5528
Elektronische ISSN: 1572-9028
DOI
https://doi.org/10.1007/s11244-013-0136-9

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