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22.07.2019 | Original Research

Effect of nickel loading approaches on the structure and hydrodeoxygenation performance of Ni/Al-SBA-15

verfasst von: Xiangping Li, Juping Liu, Jianguang Zhang, Bin Liu, Wenchao Ma, Chuanbin Wang, Guanyi Chen

Erschienen in: Cellulose | Ausgabe 15/2019

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Abstract

Lignocellulosic biomass-derived bio-oil is considered as a promising renewable biofuel. In this paper, incipient wetness impregnation method, ammonia grafting method and direct synthesis method were employed as nickel loading methods for the preparation of Ni/Al-SBA-15 catalysts. The effects of these nickel loading approaches on the structure and hydrodeoxygenation performance of Ni/Al-SBA-15 were studied. The structure of Ni/Al-SBA-15 was significantly influenced by the nickel loading methods, including the specific surface area, the pore volume, the wall thickness and so on. Nickel loading methods also affected the actual nickel content of nickel-based catalysts. Unsuccessful loading of nickel species was observed during the preparation of Ni/Al-SBA-15 using direct synthesis method. The conversion of eugenol and selectivity of products after hydrodeoxygenation in n-dodecane over Ni/Al-SBA-15 catalysts were investigated. Results showed that the conversion of eugenol nearly reached 100% for all the reaction, but the composition of product was significantly different when using different Ni/Al-SBA-15 as hydrodeoxygenation catalyst. The reaction pathway of eugenol hydrodeoxygenation in n-dodecane was also speculated in this paper.

Graphic Abstract

Effects of nickel loading approaches on the structure and hydrodeoxygenation performance of Ni/Al-SBA-15 were investigated. For the liquid phase hydrodeoxygenation of eugenol to hydrocarbon, catalysts prepared by ammonia grafting method exhibited the highest catalytic activity.

Vorheriger Artikel Ce modified Cu/Zn/Al catalysts for direct liquefaction of microcrystalline cellulose in supercritical methanol

Nächster Artikel A kinetic study on the hydrolysis of corncob residues to levulinic acid in the FeCl3–NaCl system

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Titel: Effect of nickel loading approaches on the structure and hydrodeoxygenation performance of Ni/Al-SBA-15
verfasst von: Xiangping Li
Juping Liu
Jianguang Zhang
Bin Liu
Wenchao Ma
Chuanbin Wang
Guanyi Chen
Publikationsdatum: 22.07.2019
Verlag: Springer Netherlands
Erschienen in: Cellulose / Ausgabe 15/2019
Print ISSN: 0969-0239
Elektronische ISSN: 1572-882X
DOI: https://doi.org/10.1007/s10570-019-02636-1

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