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13.11.2021 | Original Research

Enhanced hydrogen evolution under visible light by a ternary composite photocatalyst made of CdS and MoS₂ modified with bacterial cellulose aerogel

verfasst von: Lei Jiang, Mengying Xu, Shan Jiang, Pier-Luc Tremblay, Tian Zhang

Erschienen in: Cellulose | Ausgabe 1/2022

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Abstract

Heterostructure photocatalysts are developed for H₂ production from visible light. Because of their excellent photocatalytic hydrogen evolution (PHE), PCs made of CdS and MoS₂ have been studied extensively. Important characteristics of PCs to maximize PHE are efficient charge transfer and high surface area. Bacterial cellulose (BC), which is produced at a large scale from wastes of the food industry, is a promising eco-friendly candidate to improve the surface area of PCs. Here, intact BC aerogel combined with MoS₂ was added to CdS to form a ternary PC. CdS/BC-MoS₂, synthesized via a low-toxicity process, exhibited a surface area enhanced 1.5 times as well as improved photoinduced charge separation. Structural analyses demonstrated strong interactions between CdS, MoS₂, and BC in the composite PC, which was also more proficient at absorbing visible light. The PHE rate of CdS/10%BC-MoS₂ of 20.02 mmol g⁻¹ h⁻¹ was 17.7, 12.4, and 2.8 times faster than CdS, CdS with 10% BC, and CdS with 10% MoS₂, respectively. CdS/10%BC-MoS₂ exhibited an excellent quantum efficiency of 56.29%. Additionally, CdS/10%BC-MoS₂ was highly stable under visible light. These results demonstrate that BC is a suitable material to improve the performance and increase the sustainability of CdS-based heterostructure PCs.

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Vorheriger Artikel A new approach to increasing the equilibrium swelling ratio of the composite superabsorbents based on carboxymethyl cellulose sodium salt

Nächster Artikel The effects of cotton cellulose on both energy band gap of g-C3N4–TiO2 nanoparticles and enhanced photocatalytic properties of cotton-g-C3N4–TiO2 composites

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Titel: Enhanced hydrogen evolution under visible light by a ternary composite photocatalyst made of CdS and MoS2 modified with bacterial cellulose aerogel
verfasst von: Lei Jiang
Mengying Xu
Shan Jiang
Pier-Luc Tremblay
Tian Zhang
Publikationsdatum: 13.11.2021
Verlag: Springer Netherlands
Erschienen in: Cellulose / Ausgabe 1/2022
Print ISSN: 0969-0239
Elektronische ISSN: 1572-882X
DOI: https://doi.org/10.1007/s10570-021-04284-w

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