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Journal of Materials Science
Erschienen in: Journal of Materials Science 17/2016

31.05.2016 | Original Paper

Enhanced removal capability of kaolin toward methylene blue by mussel-inspired functionalization

verfasst von: Qiang Huang, Meiying Liu, Junyu Chen, Ke Wang, Dazhuang Xu, Fengjie Deng, Hongye Huang, Xiaoyong Zhang, Yen Wei

Erschienen in: Journal of Materials Science | Ausgabe 17/2016

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Abstract

Adsorption is an effective and commonly adopted method for removal of organic pollutants from environment. In this work, we described the synthesis and the adsorption behavior of poly(sodium p-styrenesulfonate hydrate) (PSPSH)-modified kaolin, which was obtained by combination of mussel-inspired chemistry and Michael addition reaction. The amino-terminated PSPSH was synthesized by free radical polymerization using cysteamine hydrochloride as the chain transfer agent and sodium p-styrenesulfonate hydrate as the monomer. Raw kaolin and PSPSH-modified kaolin were characterized using several techniques including transmission electron microscopy, Fourier transform infrared spectroscopy, thermal gravimetric analysis, and X-ray photoelectron spectroscopy in detail. The adsorption of methylene blue onto modified kaolin from aqueous solution was investigated, in which the effects of contact time, temperature, solution pH, and initial methylene blue concentration were studied. The experiment data were analyzed using two common adsorption models: Langmuir and Freundlich isotherm models. The kinetic adsorption data were analyzed using pseudo-first-order, pseudo-second-order, and intraparticle diffusion model. The values of thermodynamics constants such as entropy change (ΔS 0), enthalpy change (ΔH 0) and Gibbs free energy (ΔG 0) were also determined. The modified kaolin showed favorable dispersibility and convenient separation, high efficiency, and good regeneration capability in the removal of methylene blue from solution.
Vorheriger Artikel Herbages-derived fluorescent carbon dots and CdTe/carbon ensembles for patterning
Nächster Artikel On the transient out-of-plane behaviour of high-density cellulose-based fibre mats

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Metadaten
Titel
Enhanced removal capability of kaolin toward methylene blue by mussel-inspired functionalization
verfasst von
Qiang Huang
Meiying Liu
Junyu Chen
Ke Wang
Dazhuang Xu
Fengjie Deng
Hongye Huang
Xiaoyong Zhang
Yen Wei
Publikationsdatum
31.05.2016
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 17/2016
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-016-0082-6

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