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Environmental Earth Sciences

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01.08.2015 | Original Article

Evaluation of phosphate fertilizers and red mud in reducing plant availability of Cd, Pb, and Zn in mine tailings

verfasst von: Jun-Young Ahn, Sin-Hyun Kang, Kyung-Yup Hwang, Hong-Seok Kim, Jae-Gon Kim, Hocheol Song, Inseong Hwang

Erschienen in: Environmental Earth Sciences | Ausgabe 3/2015

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Abstract

Mono-potassium phosphate (MKP), natural phosphate fertilizer, and red mud (RM) were tested individually and as mixed agents for stabilizing Cd, Pb, and Zn in mine tailings. The mixed stabilizer containing MKP/RM was the most effective among the tested stabilizers. This is based on the efficiency of conversion from the plant-available metal fractions to the non-plant-available metal fractions and on the performances of toxicity characteristic leaching procedure tests. MKP/RM converted Cd and Zn mainly to carbonate and Fe/Mn oxide fractions, and Pb mainly to the residual fraction. When the mine tailings were treated with MKP/RM, the pH value of the stabilized soil increased from 3.4 to 6.4 after 28 days, which is advantageous for plant growth. The X-ray diffraction, scanning electron microscopy/energy dispersive spectroscopy, and the sequential extraction results imply that the major stabilization mechanism for Cd and Zn by MKP and RM involves the formation of surface complexes with Fe (hydr)oxides or Fe phosphates. The major stabilization mechanism of Pb by MKP is believed to involve the formation of Pb-phosphate precipitates, and that by RM is proposed to involve the formation of inner sphere complexes with Fe/Al (hydr)oxides or incorporation within the grids of Fe/Al (hydr)oxides or silicate minerals.

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Titel: Evaluation of phosphate fertilizers and red mud in reducing plant availability of Cd, Pb, and Zn in mine tailings
verfasst von: Jun-Young Ahn
Sin-Hyun Kang
Kyung-Yup Hwang
Hong-Seok Kim
Jae-Gon Kim
Hocheol Song
Inseong Hwang
Publikationsdatum: 01.08.2015
Verlag: Springer Berlin Heidelberg
Erschienen in: Environmental Earth Sciences / Ausgabe 3/2015
Print ISSN: 1866-6280
Elektronische ISSN: 1866-6299
DOI: https://doi.org/10.1007/s12665-015-4286-x

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