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Journal of Polymer Research

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01.09.2022 | Original Paper

Improving thermal conductivity of polyvinylidene fluoride/low-melting-point alloy with segregated structure induced by incorporation of silver interface layer

verfasst von: Ping Zhang, Xian Zhang, Xin Ding, Yanyan Wang, Chao Xiao, Kang Zheng, Lin Chen, Xingyou Tian

Erschienen in: Journal of Polymer Research | Ausgabe 9/2022

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Abstract

Low-melting-point alloy (LMPA) is regarded as one of the most promising fillers for improving heat dissipation performance of polymer-matrix composites. Nevertheless, the promise of excellent functional composites with low content of LMPA has been greatly weakened as poor compatibility between LMPA and polymer. To address this problem, introducing metal interface layer to polymer microsphere’ surface is promising method by inspiration of depositing silver coating on copper-clad laminates. Here, silver interface layer was introduced to the surface of polyvinylidene fluoride microspheres through the polydopamine (PVDF@PDA@Ag). After mixing PVDF@PDA@Ag microspheres with Sn-58Bi (LMPA), PVDF@PDA@Ag/LMPA composite with segregated structure was successfully fabricated by hot-pressing. X-ray diffraction (XRD) test revealed that intermetallic compounds of Ag₃Sn was production. Owing to Ag₃Sn promoting LMPA coated on surface of microsphere, the microscopic conduction path of composites transforming from irregular continuous LMPA network to segregated network. In the case of low LMPA content (10 vol%), PVDF@PDA@Ag/LMPA composite owned thermal conductivity of 1.79 W/mK, while PVDF/LMPA composite was only 0.36 W/mK. Compared to PVDF/LMPA composite, the enhancement factor of PVDF@PDA@Ag/LMPA composite was improved from 56.52% to 678.26%. This article offered viable route to enhance compatibility between polymer and LMPA.

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Nächster Artikel On the characterization of viscoelastic behaviours of ultra-high molecular polyethylene composite with 1-ethyl-3-methylimidazolium ethyl sulfate ionic liquid

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Titel: Improving thermal conductivity of polyvinylidene fluoride/low-melting-point alloy with segregated structure induced by incorporation of silver interface layer
verfasst von: Ping Zhang
Xian Zhang
Xin Ding
Yanyan Wang
Chao Xiao
Kang Zheng
Lin Chen
Xingyou Tian
Publikationsdatum: 01.09.2022
Verlag: Springer Netherlands
Erschienen in: Journal of Polymer Research / Ausgabe 9/2022
Print ISSN: 1022-9760
Elektronische ISSN: 1572-8935
DOI: https://doi.org/10.1007/s10965-022-03242-9

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