Skip to main content
Erschienen in: Environmental Earth Sciences 7/2015

01.04.2015 | Original Article

Leachability of phenanthrene from soil under acid rain and its relationship with dissolved organic matter

verfasst von: Wenjie Tian, Lijian Wang, Dong Li, Fasheng Li

Erschienen in: Environmental Earth Sciences | Ausgabe 7/2015

Einloggen

Aktivieren Sie unsere intelligente Suche, um passende Fachinhalte oder Patente zu finden.

search-config
loading …

Abstract

Acid rain is a serious environmental problem in the world. Soil columns were leached with simulated acid rain (SAR) at pH ranging from 2.5 to 5.6. The impact of SAR on the release of phenanthrene from red soil and its correlation with dissolved organic carbon (DOC) in eluates were investigated. The results showed that the leaching loss of phenanthrene was affected by both the leaching volume and acidity of SAR. When the leaching volume was less than 500 mm, the phenanthrene concentration in eluates decreased rapidly with increasing leaching volume, indicating a high rate of leaching loss at the beginning of leaching; then with continuous leaching, the phenanthrene concentration decreased slightly and reached zero when the leaching volume reached 875 mm. The lower pH of SAR was, the higher release rate of phenanthrene was. The change of DOC in eluates was similar to that of the phenanthrene concentration. The phenanthrene concentration had a significantly positive correlation with DOC in all eluates (the squared correlation coefficient R 2 varied between 0.952 and 0.997). Three-dimensional fluorescence analysis revealed that phenanthrene was associated with humic acid and fulvic acid, and was released with dissolved organic matters leached by SAR.

Sie haben noch keine Lizenz? Dann Informieren Sie sich jetzt über unsere Produkte:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

Anhänge
Nur mit Berechtigung zugänglich
Literatur
Zurück zum Zitat Calace N, Fiorentini F, Petronio BM, Pietroletti M (2001) Effects of acid rain on soil humic compounds. Talanta 54:837–846CrossRef Calace N, Fiorentini F, Petronio BM, Pietroletti M (2001) Effects of acid rain on soil humic compounds. Talanta 54:837–846CrossRef
Zurück zum Zitat Chen J, LeBoeuf EJ, Dai S, Gu B (2003a) Fluorescence spectroscopic studies of natural organic matter fractions. Chemosphere 50:639–647CrossRef Chen J, LeBoeuf EJ, Dai S, Gu B (2003a) Fluorescence spectroscopic studies of natural organic matter fractions. Chemosphere 50:639–647CrossRef
Zurück zum Zitat Chen W, Westerhoff P, Leenheer JA, Booksh K (2003b) Fluorescence excitation–emission matrix regional integration to quantify spectra for dissolved organic matter. Environ Sci Technol 37:5701–5710CrossRef Chen W, Westerhoff P, Leenheer JA, Booksh K (2003b) Fluorescence excitation–emission matrix regional integration to quantify spectra for dissolved organic matter. Environ Sci Technol 37:5701–5710CrossRef
Zurück zum Zitat Cooke CM, Shaw G, Collins CD (2004) Determination of solid–liquid partition coefficients (Kd) for the herbicides isoproturon and trifluralin in five UK agricultural soils. Environ Pollut 132:541–552CrossRef Cooke CM, Shaw G, Collins CD (2004) Determination of solid–liquid partition coefficients (Kd) for the herbicides isoproturon and trifluralin in five UK agricultural soils. Environ Pollut 132:541–552CrossRef
Zurück zum Zitat Cox L, Celis R, Hermosin MC, Cornejo J, Zsolnay A, Zeller K (2000) Effect of organic amendments on herbicide sorption as related to the nature of the dissolved organic matter. Environ Sci Technol 34:4600–4605CrossRef Cox L, Celis R, Hermosin MC, Cornejo J, Zsolnay A, Zeller K (2000) Effect of organic amendments on herbicide sorption as related to the nature of the dissolved organic matter. Environ Sci Technol 34:4600–4605CrossRef
Zurück zum Zitat Gan S, Lau EV, Ng HK (2009) Remediation of soils contaminated with polycyclic aromatic hydrocarbons (PAHs). J Hazard Mater 172:532–549CrossRef Gan S, Lau EV, Ng HK (2009) Remediation of soils contaminated with polycyclic aromatic hydrocarbons (PAHs). J Hazard Mater 172:532–549CrossRef
Zurück zum Zitat Gao YZ, Zhu LZ (2004) Plant uptake accumulation and translocation of phenanthrene and pyrene in soils. Chemosphere 55:1169–1178CrossRef Gao YZ, Zhu LZ (2004) Plant uptake accumulation and translocation of phenanthrene and pyrene in soils. Chemosphere 55:1169–1178CrossRef
Zurück zum Zitat Gao YZ, Xiong W, Ling WT, Wang XR, Li QL (2007) Impact of exotic and inherent dissolved organic matter on sorption of phenanthrene by soils. J Hazard Mater 140:138–144CrossRef Gao YZ, Xiong W, Ling WT, Wang XR, Li QL (2007) Impact of exotic and inherent dissolved organic matter on sorption of phenanthrene by soils. J Hazard Mater 140:138–144CrossRef
Zurück zum Zitat He YW, Ou ZQ, Sun TH (1995) Adsorption of polycyclic aromatic hydrocarbons on soil. J Appl Ecol 6:423–427CrossRef He YW, Ou ZQ, Sun TH (1995) Adsorption of polycyclic aromatic hydrocarbons on soil. J Appl Ecol 6:423–427CrossRef
Zurück zum Zitat Jones KD, Tiller CL (1999) Effect of solution chemistry on the extent of binding of phenanthrene by a soil humic acid: a comparison of dissolved and clay bound humic acids. Environ Sci Technol 33:580–587CrossRef Jones KD, Tiller CL (1999) Effect of solution chemistry on the extent of binding of phenanthrene by a soil humic acid: a comparison of dissolved and clay bound humic acids. Environ Sci Technol 33:580–587CrossRef
Zurück zum Zitat Kohl SD, Rice JA (1998) The binding of contaminants to humin: a mass balance. Chemosphere 36:251–261CrossRef Kohl SD, Rice JA (1998) The binding of contaminants to humin: a mass balance. Chemosphere 36:251–261CrossRef
Zurück zum Zitat Krauss M, Wilcke W (2002) Sorption strength of persistent organic pollutants in particle-size fractions of urban soils. Soil Sci Soc Am J 66:430–437CrossRef Krauss M, Wilcke W (2002) Sorption strength of persistent organic pollutants in particle-size fractions of urban soils. Soil Sci Soc Am J 66:430–437CrossRef
Zurück zum Zitat Lapenis AG, Lawrence GB, Andreev AA et al (2004) Acidification of forest soil in Russia: from 1893 to present. Global Biogeochem Cyc 18:1–13CrossRef Lapenis AG, Lawrence GB, Andreev AA et al (2004) Acidification of forest soil in Russia: from 1893 to present. Global Biogeochem Cyc 18:1–13CrossRef
Zurück zum Zitat Larssen T, Carmichael GR (2000) Acid rain and acidification in China: the importance of base cation deposition. Environ Pollut 110:89–102CrossRef Larssen T, Carmichael GR (2000) Acid rain and acidification in China: the importance of base cation deposition. Environ Pollut 110:89–102CrossRef
Zurück zum Zitat Larssen T, Lydersen E, Tang D (2006) Acid rain in China: rapid industrialization has put citizens and ecosystems at risk. Environ Sci Technol 40:418–425CrossRef Larssen T, Lydersen E, Tang D (2006) Acid rain in China: rapid industrialization has put citizens and ecosystems at risk. Environ Sci Technol 40:418–425CrossRef
Zurück zum Zitat Liu L, Song CY, Yan ZG, Li FS (2009) Characterizing the release of different composition of dissolved organic matter in soil under acid rain leaching using three-dimensional excitation–emission matrix spectroscopy. Chemosphere 77:15–21CrossRef Liu L, Song CY, Yan ZG, Li FS (2009) Characterizing the release of different composition of dissolved organic matter in soil under acid rain leaching using three-dimensional excitation–emission matrix spectroscopy. Chemosphere 77:15–21CrossRef
Zurück zum Zitat Means JC, Wood SG, Hassett JJ, Banwart WL (1980) Sorption of polynuclear aromatic hydrocarbons by sediments and soils. Environ Sci Technol 1:1524–1528CrossRef Means JC, Wood SG, Hassett JJ, Banwart WL (1980) Sorption of polynuclear aromatic hydrocarbons by sediments and soils. Environ Sci Technol 1:1524–1528CrossRef
Zurück zum Zitat Menon M, Hermle S, Gunthardt-Goerg MS et al (2007) Effects of heavy metal soil pollution and acid rain on growth and water use efficiency of a young model forest ecosystem. Plant Soil 297:171–183CrossRef Menon M, Hermle S, Gunthardt-Goerg MS et al (2007) Effects of heavy metal soil pollution and acid rain on growth and water use efficiency of a young model forest ecosystem. Plant Soil 297:171–183CrossRef
Zurück zum Zitat Nemeth-Konda L, Gy Morovjan, Csokan P (2002) Sorption behaviour of acetochlor, atrazine, carbendazim, diazinon imidacloprid and isoproturon on Hungarian agricultural soil. Chemosphere 48:545–552CrossRef Nemeth-Konda L, Gy Morovjan, Csokan P (2002) Sorption behaviour of acetochlor, atrazine, carbendazim, diazinon imidacloprid and isoproturon on Hungarian agricultural soil. Chemosphere 48:545–552CrossRef
Zurück zum Zitat Ni JZ, Luo YM, Wei R, Li XH (2008) Distribution patterns of polycyclic aromatic hydrocarbons among different organic carbon fractions of polluted agricultural soils. Geoderma 146:277–282CrossRef Ni JZ, Luo YM, Wei R, Li XH (2008) Distribution patterns of polycyclic aromatic hydrocarbons among different organic carbon fractions of polluted agricultural soils. Geoderma 146:277–282CrossRef
Zurück zum Zitat NSCO (National Soil Census Office) (1998) Soil of China. Agricultural Press, Beijing (in Chinese) NSCO (National Soil Census Office) (1998) Soil of China. Agricultural Press, Beijing (in Chinese)
Zurück zum Zitat Pan B, Xing BS, Tao S (2007) Effect of physical forms of soil organic matter on phenanthrene sorption. Chemosphere 68:1262–1269CrossRef Pan B, Xing BS, Tao S (2007) Effect of physical forms of soil organic matter on phenanthrene sorption. Chemosphere 68:1262–1269CrossRef
Zurück zum Zitat Parrish ZD, Banks MK, Schwab AP (2005) Assessment of contaminant liability during phytoremediation of polycyclic aromatic hydrocarbon impacted soil. Environ Pollut 137:187–197CrossRef Parrish ZD, Banks MK, Schwab AP (2005) Assessment of contaminant liability during phytoremediation of polycyclic aromatic hydrocarbon impacted soil. Environ Pollut 137:187–197CrossRef
Zurück zum Zitat Qi WQ, Xi JQ, Wang ZG (2002) The actuality and trend of acid rain research. Environ Monit 18:7–11 Qi WQ, Xi JQ, Wang ZG (2002) The actuality and trend of acid rain research. Environ Monit 18:7–11
Zurück zum Zitat Ross DS, Bartlett RJ (1996) Field extracted spodosol solutions and soils: aluminum, organic carbon and pH relationships. Soil Sci Soc Am J 60:589–595CrossRef Ross DS, Bartlett RJ (1996) Field extracted spodosol solutions and soils: aluminum, organic carbon and pH relationships. Soil Sci Soc Am J 60:589–595CrossRef
Zurück zum Zitat Simpson MJ, Chefetz B, Hatcher PG (2003) Phenanthrene sorption to structurally modified humic acids. J Environ Qual 32:1750–1758CrossRef Simpson MJ, Chefetz B, Hatcher PG (2003) Phenanthrene sorption to structurally modified humic acids. J Environ Qual 32:1750–1758CrossRef
Zurück zum Zitat Sojinu OS, Wang JZ, Sonibare OO (2010) Polycyclic aromatic hydrocarbons in sediments and soils from oil exploration areas of the Niger Delta, Nigeria. J Hazard Mater 174:641–647CrossRef Sojinu OS, Wang JZ, Sonibare OO (2010) Polycyclic aromatic hydrocarbons in sediments and soils from oil exploration areas of the Niger Delta, Nigeria. J Hazard Mater 174:641–647CrossRef
Zurück zum Zitat Stemmer M, Watzinger A, Blochberger K (2007) Linking dynamics of soil microbial phospholipid fatty acids to carbon mineralization in a C-13 natural abundance experiment: impact of heavy metals and acid rain. Soil Biol Biochem 39:3177–3186CrossRef Stemmer M, Watzinger A, Blochberger K (2007) Linking dynamics of soil microbial phospholipid fatty acids to carbon mineralization in a C-13 natural abundance experiment: impact of heavy metals and acid rain. Soil Biol Biochem 39:3177–3186CrossRef
Zurück zum Zitat Tao FL, Feng ZW (2000) Soil sensitivity to acid deposition in south China. Acta Sci Circumstantiae 20:126–128 (in Chinese) Tao FL, Feng ZW (2000) Soil sensitivity to acid deposition in south China. Acta Sci Circumstantiae 20:126–128 (in Chinese)
Zurück zum Zitat Tejada M, Gonzalez JL (2007) Influence of organic amendments on soil structure and soil loss under simulated rain. Soil Till Res 93:197–205CrossRef Tejada M, Gonzalez JL (2007) Influence of organic amendments on soil structure and soil loss under simulated rain. Soil Till Res 93:197–205CrossRef
Zurück zum Zitat Wang LF, Pan GX, Shi SL, Huang MX, Zhang LX (2002) Dissolved organic carbon in soil solution of paludalfs udalfsin Mt. Lushan forest under impact of acid deposition. J Plant Nutr Soil Sci 8:29–34 (in Chinese) Wang LF, Pan GX, Shi SL, Huang MX, Zhang LX (2002) Dissolved organic carbon in soil solution of paludalfs udalfsin Mt. Lushan forest under impact of acid deposition. J Plant Nutr Soil Sci 8:29–34 (in Chinese)
Zurück zum Zitat Weng L, Temminghoff EJ, Van Riemsdijk WH (2002) Interpretation of humic acid coagulation and soluble soil organic matter using a calculated electrostatic potential. Euro J Soil Sci 53:575–588CrossRef Weng L, Temminghoff EJ, Van Riemsdijk WH (2002) Interpretation of humic acid coagulation and soluble soil organic matter using a calculated electrostatic potential. Euro J Soil Sci 53:575–588CrossRef
Zurück zum Zitat Wu FC, Wu JW, Wang XY, Zou J (2000) Study on acid rain pollution in Hunan province. Acta Sci Circumstantiae 20:807–809 (in Chinese) Wu FC, Wu JW, Wang XY, Zou J (2000) Study on acid rain pollution in Hunan province. Acta Sci Circumstantiae 20:807–809 (in Chinese)
Zurück zum Zitat Xu ZJ, Liu GS, Yu JD, Liu W (2002) Effects of acid rain on aggregate and it’s cemedins of red soil by simulated experiments. J Soil Water Conserv 16:9–11 Xu ZJ, Liu GS, Yu JD, Liu W (2002) Effects of acid rain on aggregate and it’s cemedins of red soil by simulated experiments. J Soil Water Conserv 16:9–11
Zurück zum Zitat Yang Y, Tao S, Zhang N, Zhang DY, Li XQ (2010a) The effect of soil organic matter on fate of polycyclic aromatic hydrocarbons in soil: a microcosm study. Environ Pollut 158:1768–1774CrossRef Yang Y, Tao S, Zhang N, Zhang DY, Li XQ (2010a) The effect of soil organic matter on fate of polycyclic aromatic hydrocarbons in soil: a microcosm study. Environ Pollut 158:1768–1774CrossRef
Zurück zum Zitat Yang Y, Zhang N, Xue M, Tao S (2010b) Impact of soil organic matter on the distribution of polycyclic aromatic hydrocarbons (PAHs) in soils. Environ Pollut 158:2170–2174CrossRef Yang Y, Zhang N, Xue M, Tao S (2010b) Impact of soil organic matter on the distribution of polycyclic aromatic hydrocarbons (PAHs) in soils. Environ Pollut 158:2170–2174CrossRef
Zurück zum Zitat Zhang MK, Calvert DV (2005) Simulation study on copper and zinc release from contaminated sandy soils due to acidification. J Forest Res 16:289–292CrossRef Zhang MK, Calvert DV (2005) Simulation study on copper and zinc release from contaminated sandy soils due to acidification. J Forest Res 16:289–292CrossRef
Zurück zum Zitat Zhang JE, Ouyang Y, Ling DJ (2007) Impacts of simulated acid rain on cation leaching from the Latosol in south China. Chemosphere 67:2131–2137CrossRef Zhang JE, Ouyang Y, Ling DJ (2007) Impacts of simulated acid rain on cation leaching from the Latosol in south China. Chemosphere 67:2131–2137CrossRef
Metadaten
Titel
Leachability of phenanthrene from soil under acid rain and its relationship with dissolved organic matter
verfasst von
Wenjie Tian
Lijian Wang
Dong Li
Fasheng Li
Publikationsdatum
01.04.2015
Verlag
Springer Berlin Heidelberg
Erschienen in
Environmental Earth Sciences / Ausgabe 7/2015
Print ISSN: 1866-6280
Elektronische ISSN: 1866-6299
DOI
https://doi.org/10.1007/s12665-014-3653-3

Weitere Artikel der Ausgabe 7/2015

Environmental Earth Sciences 7/2015 Zur Ausgabe