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Journal of Materials Science

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23.08.2022 | Energy materials

A combinatorial improvement strategy to enhance the energy storage performances of the KNN–based ferroelectric ceramic capacitors

verfasst von: Lingzhi Wu, Yu Huan, Xinjian Wang, Changxiao Li, Ying Luo, Tao Wei

Erschienen in: Journal of Materials Science | Ausgabe 33/2022

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Abstract

With the increasing demand for miniaturization and integration in electronic equipment, environmental-friendly K_0.5Na_0.5NbO₃ (KNN) based lead–free energy storage ceramic capacitors have caused extensive concern not only for their ultrahigh power density but also for ultrafast charging/discharging rates. However, their recoverable energy storage density (W_rec) and efficiency (η) are poor due to the large energy loss (W_loss) and low breakdown electric field (E_b). In this work, a combinatorial improvement strategy is proposed to enhance the energy storage performance of KNN–based ceramics. First, the introduction of 0.05Bi(Zn_0.5(Ti_1–xZr_x)_0.5)O₃ (BZTZ) solid solution in pure KNN ceramics extremely destroys the long–range polar ordering and forms the PNRs, which effectively decreases the remnant polarization (P_r) and enhances η. Second, the substitution of Zr to Ti ions reduces the migration of grain boundary and thereby inhibits grain growth. Third, the BZTZ solid solution as a high–κ insulator improves the band–gap energy (E_g) of the KNN–based ceramics. Both of them could boost E_b. Finally, the x = 0.75 ceramic with an excellent W_rec (3.70 J cm^–3) and η (75.3%) at a particularly large E_b (340 kV cm^–1) was successfully obtained. The combinatorial improvement strategy in this work provides a novel way to enhance the energy storage performance of the lead–free dielectric capacitors.

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Vorheriger Artikel Effect of Nb doping on epsilon negative behaviour of Sr2MnO4

Nächster Artikel Magnetron sputtered Al-doped NiOx films as a hole transport layer for perovskite solar cells

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Titel: A combinatorial improvement strategy to enhance the energy storage performances of the KNN–based ferroelectric ceramic capacitors
verfasst von: Lingzhi Wu
Yu Huan
Xinjian Wang
Changxiao Li
Ying Luo
Tao Wei
Publikationsdatum: 23.08.2022
Verlag: Springer US
Erschienen in: Journal of Materials Science / Ausgabe 33/2022
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI: https://doi.org/10.1007/s10853-022-07554-5

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