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Journal of Materials Science
Erschienen in: Journal of Materials Science 17/2018

30.05.2018 | Energy materials

Biomass-based O, N-codoped activated carbon aerogels with ultramicropores for supercapacitors

verfasst von: Zhengqing Ye, Feijun Wang, Chao Jia, Ziqiang Shao

Erschienen in: Journal of Materials Science | Ausgabe 17/2018

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Abstract

Three-dimensional (3D) O, N-codoped activated carbon aerogels with ultramicropores were prepared via oxidation polymerization, freeze-drying, and carbonization/activation of aniline and sodium alginate. All the O, N-codoped activated carbon aerogels exhibit 3D interconnected hierarchical porous network structures with high specific surface areas (1337–1695 m2 g−1), ultramicropores (0.52–0.54 nm), and rich O (12.68–18.48%) and N (1.18–3.59%) doping. A typical 3D O, N-codoped activated carbon aerogel (ACA700) obtained at the activation of 700 °C exhibits excellent electrochemical performance. When ACA700 is utilized as electrode materials for supercapacitor, the highest specific capacitance of 342 F g−1 at a current density of 2 A g−1 in 3 M H2SO4 electrolyte is achieved. Furthermore, ACA700//ACA700 all-solid-state supercapacitor device displays acceptable energy density (3.8 Wh kg−1) at a power density of 246.0 W kg−1, extraordinary coulombic efficiency (95.8%), and good rate capability. Therefore, the sustainable 3D O, N-codoped activated carbon aerogels with ultramicropores demonstrate tremendous potential for energy storage devices.
Vorheriger Artikel Porous composite separator membranes of dye-sensitized solar cells with flexible substrate for their improved stability
Nächster Artikel Amorphous molybdenum sulphide @ nanoporous gold as catalyst for hydrogen evolution reaction in acidic environment

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Metadaten
Titel
Biomass-based O, N-codoped activated carbon aerogels with ultramicropores for supercapacitors
verfasst von
Zhengqing Ye
Feijun Wang
Chao Jia
Ziqiang Shao
Publikationsdatum
30.05.2018
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 17/2018
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-018-2487-x

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