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Journal of Materials Science
Erschienen in: Journal of Materials Science 26/2021

14.06.2021 | Energy materials

Enhanced dielectric temperature stability and energy-storage properties of (Y0.5Nb0.5)4+ co-doped (Bi0.5Na0.5)0.94Ba0.06TiO3 lead-free relaxor ceramics

verfasst von: Han Wang, Qiang Li, Yuxin Jia, Arun Kumar Yadav, Benben Yan, Qi Shen, Mengyuan Li, Qifeng Quan, Huiqing Fan

Erschienen in: Journal of Materials Science | Ausgabe 26/2021

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Abstract

(Bi0.5Na0.5)0.94Ba0.06Ti1−x(Y0.5Nb0.5)xO3 (abbreviated as BNTBT-100xYN) lead-free relaxor ceramics were designed and prepared using a traditional solid-state sintering technique. The influences of the introduction of (Y0.5Nb0.5)4+ complex ions for the dielectric properties and energy storage performances of BNTBT-100xYN ceramics were systematically studied. All samples exhibited a typical pseudo-cubic symmetry structure and obtained the dense microstructure with the uniform distribution of all elements. The ergodic relaxor behavior of all ceramics was observed and revealed a trend of increase as a function of composition. It accelerated the improvement of the temperature stability of the dielectric constant. All samples showed a single grain conduction mechanism and the activation energy decreased with the addition of composition. It is related to the generation of oxygen vacancies induced by the defect dipoles. BNTBT-6YN ceramic revealed excellent dielectric temperature stability within the temperature range from 87 to 479 °C and the loss tangent less than 0.05 between 25 °C and 474 °C. Besides, a high recoverable energy density of ~ 0.91 J/cm3 with the corresponding efficiency of ~ 78.5% at applied 115 kV/cm field was achieved for BNTBT-5YN ceramic. Hence, BNTBT-5YN and BNTBT-6YN ceramics will become one of the outstanding dielectric ceramics for the electronic components.
Vorheriger Artikel TiO2-x nanoparticles dispersed in center-radial channels of dendritic mesoporous silica nanospheres (DMSNs) as novelly structured photocatalysts
Nächster Artikel Ni-Zn supported defective carbon with multi-functional catalytic sites for Baeyer–Villiger reaction using air as oxidant

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Metadaten
Titel
Enhanced dielectric temperature stability and energy-storage properties of (Y0.5Nb0.5)4+ co-doped (Bi0.5Na0.5)0.94Ba0.06TiO3 lead-free relaxor ceramics
verfasst von
Han Wang
Qiang Li
Yuxin Jia
Arun Kumar Yadav
Benben Yan
Qi Shen
Mengyuan Li
Qifeng Quan
Huiqing Fan
Publikationsdatum
14.06.2021
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 26/2021
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-021-06193-6

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