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Journal of Materials Science
Erschienen in: Journal of Materials Science 29/2023

24.07.2023 | Ceramics

Capacitive energy storage performance of lead-free sodium niobate-based antiferroelectric ceramics

verfasst von: Ye Lu, Ji Zhang, Kedong Zhou, Lei He

Erschienen in: Journal of Materials Science | Ausgabe 29/2023

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Abstract

Ceramic-based capacitors have attracted great interest due to their large power density and ultrafast charge/discharge time, which are needful properties for pulsed-power devices. Antiferroelectric ceramics normally show ultrahigh energy density and relatively low efficiency, which is ascribed to the electric field-induced antiferroelectric–ferroelectric phase transition. This work reports that the perovskite end-member Bi(Fe1/3Zn1/3Ti1/3)O3 is added into NaNbO3 lead-free antiferroelectric ceramics. The lower tolerance factor of Bi(Fe1/3Zn1/3Ti1/3)O3 facilitates to achieve stable antiferroelectric phase in NaNbO3, and the introduction of various ions enhances the relaxor behavior. Consequently, the optimized 0.88NaNbO3 − 0.12Bi(Fe1/3Zn1/3Ti1/3)O3 ceramics exhibit a large recoverable energy density of 6.8 J/cm3 and a high efficiency of 82% under 49 kV/mm, as well as discharge energy density of 4 J/cm3 and charge/discharge time of 5 μs. This study suggests that the incorporation of relaxor properties into antiferroelectric ceramics is a beneficial route to boost the dielectric energy storage capability.
Vorheriger Artikel Transparent Al2O3 fabricated by energy efficient spark plasma sintering
Nächster Artikel Solvothermal synthesis of nanostructured nickel-based metal–organic frameworks (Ni-MOFs) with enhanced electrochemical performance for symmetric supercapacitors

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Metadaten
Titel
Capacitive energy storage performance of lead-free sodium niobate-based antiferroelectric ceramics
verfasst von
Ye Lu
Ji Zhang
Kedong Zhou
Lei He
Publikationsdatum
24.07.2023
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 29/2023
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-023-08769-w

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