Natural and artificial radioactivity distribution in soil, rock and water of the Central Ashanti Gold Mine, Ghana

Direct gamma spectrometry study was carried out within and around the operational area of the Central Ashanti Gold of Ghana to ascertain the baseline radioactivity levels of naturally occurring radioactive materials (NORM), prior to processing of gold ore at the mine. The average activity concentrations of ²³⁸U, ²³²Th, ⁴⁰K and ¹³⁷Cs in the soil/rock samples were 64.3, 68.4, 1243.9 and 3.5 Bqkg⁻¹, respectively. For the water samples, the average activity concentrations were 2.5, 2.6, 14.7 and 0.7 BqL⁻¹ for ²³⁸U, ²³²Th, ⁴⁰K and ¹³⁷Cs, respectively. The total annual effective dose to the public was estimated to be 0.141 mSv which is below the ICRP recommended level of 1 mSv for public exposure control. The average radium equivalent activity value was 257.8 Bqkg⁻¹ in the range of 72.9–402.3 Bqkg⁻¹. The average values of external and internal indices were 0.7 and 0.8, respectively. The concentrations of U, Th and K were variable in soil and rock samples taken from different locations in the study area with values varying in the range of 0.8–10.9, 2.4–39.4 μg/g and 0.7–6.3 %, respectively. The concentration values of gross-α and gross-β for all the water samples were below the Ghana Standards Board and Who Health Organisation recommended guideline values for drinking water quality. The results obtained in this study shows that radiation levels are within the natural background radiation levels found in literature and compared well with similar studies for other countries.