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Journal of Material Cycles and Waste Management
Erschienen in: Journal of Material Cycles and Waste Management 5/2019

29.05.2019 | ORIGINAL ARTICLE

Removal of Mn and Cd contained in mine wastewater by Mg–Al-layered double hydroxides

verfasst von: Mir Tamzid Rahman, Tomohito Kameda, Takao Miura, Shogo Kumagai, Toshiaki Yoshioka

Erschienen in: Journal of Material Cycles and Waste Management | Ausgabe 5/2019

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Abstract

The fate of heavy metals in the environment is significantly influenced by their adsorption onto clay minerals. Herein, we investigate the mechanism of MnO4− and Cd2+ removal by nitrate-intercalated Mg–Al-layered double hydroxides (LDHs) in aqueous solution and optimize the corresponding conditions, showing that these adsorbents can effectively remove Zn, Mn, and Cd from mine wastewater and revealing that adsorbent structure is retained after wastewater treatment. The removal of MnO4− ions from aqueous solution is demonstrated to proceed via their exchange for NO3− ions intercalated within LDHs and is well described by the Freundlich adsorption model, following pseudo-second-order kinetics and featuring chemisorption as the rate-determining step. In contrast, Cd2+ is shown to be removed via the formation of Cd5(OH)8(NO3)2·2H2O (at LDH2) and Cd(NO3)2·Cd(OH)2 (at LDH1).
Vorheriger Artikel Waste ashes as catalysts for the pyrolysis–catalytic steam reforming of biomass for hydrogen-rich gas production
Nächster Artikel Synthesis of layered double hydroxide from asbestos-containing waste and its adsorption property

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Metadaten
Titel
Removal of Mn and Cd contained in mine wastewater by Mg–Al-layered double hydroxides
verfasst von
Mir Tamzid Rahman
Tomohito Kameda
Takao Miura
Shogo Kumagai
Toshiaki Yoshioka
Publikationsdatum
29.05.2019
Verlag
Springer Japan
Erschienen in
Journal of Material Cycles and Waste Management / Ausgabe 5/2019
Print ISSN: 1438-4957
Elektronische ISSN: 1611-8227
DOI
https://doi.org/10.1007/s10163-019-00875-9

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