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Journal of Materials Science: Materials in Electronics

Erschienen in:

02.11.2020

Ultrahigh nitrogen-doped carbon/superfine-Sn particles for lithium ion battery anode

verfasst von: Han Bi, Xin Li, Jingjing Chen, Lexi Zhang, Lijian Bie

Erschienen in: Journal of Materials Science: Materials in Electronics | Ausgabe 24/2020

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Abstract

Graphitic carbon nitride (g-C₃N₄) can be indexed as a high-content N-doped carbon material, appealing great attentions in energy storage devices. However, poor conductivity and serious irreversible capacity loss were found for the g-C₃N₄ due to its high nitrogen content. Urea, dicyandiamide or melamine can be used as organic precursor to form g-C₃N₄ because they can be pyrolyzed into g-C₃N₄ easily. In this work, high nitrogen content (up to 17 at.%)-doped carbon materials embedded with superfine-Sn particle are synthesized by one-step thermal treatment of the g-C₃N₄ organic precursor and SnCl₂ in a simple self-designed quartz tube. Regarding their high nitrogen doping content, large surface area and porous structure, the obtained material could deliver a high specific capacity and excellent capacity retention when applied as lithium ion battery anode. Its excellent rate performance is attributed to the high Li diffusion coefficient demonstrated by the GITT kinetics analysis. This extremely simple and low-cost preparation process could provide a new strategy to obtain high nitrogen content carbon-based materials.

Vorheriger Artikel Synthesis and characterization of (1 − y) [0.996Na0.475K0.475Li0.05Sb0.05Nb0.95O3–0.004Bi0.95Nd0.05FeO3] + (y) [Co0.50Cu0.15Zn0.35Fe1.95Mn0.05O4] composites

Nächster Artikel A novel research on the subject of the load-independent microhardness performances of Sr/Ti partial displacement in Bi-2212 ceramics

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Titel: Ultrahigh nitrogen-doped carbon/superfine-Sn particles for lithium ion battery anode
verfasst von: Han Bi
Xin Li
Jingjing Chen
Lexi Zhang
Lijian Bie
Publikationsdatum: 02.11.2020
Verlag: Springer US
Erschienen in: Journal of Materials Science: Materials in Electronics / Ausgabe 24/2020
Print ISSN: 0957-4522
Elektronische ISSN: 1573-482X
DOI: https://doi.org/10.1007/s10854-020-04723-7

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