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Biomass Conversion and Biorefinery

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07.07.2021 | Original Article

Experimental study on the effect of water addition to ChCl-MEA DES towards its performance in CO₂ removal from syngas

verfasst von: Haryo Wibowo, Li Zhong, Qun Huan, Qing Hu, Dicka Ar Rahim, Mi Yan

Erschienen in: Biomass Conversion and Biorefinery | Sonderheft 1/2022

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Abstract

ChCl-MEA DES was used to absorb CO₂ from gasification syngas consisting of CO₂, CO, CH₄, and H₂. This study investigated the effect of water addition on CO₂ absorption capabilities of ChCl-MEA DES with different mole ratios of ChCl to MEA, and different absorption temperatures. It was found that water addition had a positive effect on CO₂ solubility of ChCl-MEA DES, with the maximum obtained value of 0.5 mol-CO₂/mol-DES for aqueous ChCl-MEA DES with 75%vol water at absorption temperature of 40 °C and pressure of 9 bar. In general, water addition increases CO₂ solubility and absorption rate of ChCl-MEA DES. ChCl-MEA DES 1:5 mol ratio was able to benefit from water addition up to 75%vol water content. While ChCl-MEA 1:10 had its CO₂ solubility increase with water addition up to 50%vol, after which, it declined. Investigation into water addition at different absorption temperatures revealed that water addition at 40 °C produced the most significant CO₂ solubility enhancement compared to water addition at 20 °C and 60 °C. This might be caused by the tradeoff between the effects of high temperature in decreasing ChCl-MEA DES viscosity and lowering its CO₂ solubility. Highest CO₂/CO selectivity for ChCl-MEA DES 1:5 was found to be around 34.6, CO₂/CH₄ was 26.7, and CO₂/H₂ was 4. Water addition was found to have slight reducing effect on the CO₂ selectivity of ChCl-MEA DES.

Vorheriger Artikel An eco-friendly and sustainable system for monitoring the oleuropein-rich extract from olive tree (Olea europaea) leaves

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Titel: Experimental study on the effect of water addition to ChCl-MEA DES towards its performance in CO2 removal from syngas
verfasst von: Haryo Wibowo
Li Zhong
Qun Huan
Qing Hu
Dicka Ar Rahim
Mi Yan
Publikationsdatum: 07.07.2021
Verlag: Springer Berlin Heidelberg
Erschienen in: Biomass Conversion and Biorefinery / Ausgabe Sonderheft 1/2022
Print ISSN: 2190-6815
Elektronische ISSN: 2190-6823
DOI: https://doi.org/10.1007/s13399-021-01673-w

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