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Journal of Materials Science: Materials in Electronics
Erschienen in: Journal of Materials Science: Materials in Electronics 3/2020

14.12.2019

MoC/MnO composite materials as high efficient and stable counter electrode catalysts for dye-sensitized solar cells

verfasst von: Aidong Peng, Yuan Gao, Qun Yang, Xueqin Zuo, Huaibao Tang, Guang Li

Erschienen in: Journal of Materials Science: Materials in Electronics | Ausgabe 3/2020

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Abstract

MoC/MnO composite materials have been easily synthesized via a two-step hydrothermal and one-step carbonization method and used as counter electrode catalysts in DSSCs for the first time. The as-prepared samples were characterized by X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), scanning electron microscopy (SEM) and transmission electron microscopy (TEM). And their electrocatalytic properties were also thoroughly studied by electrochemical impedance spectroscopy (EIS), Tafel polarization and so on. It is found that the electrocatalytic properties of the MoC/MnO CEs can be greatly enhanced. After optimizing the molar ratio of MoO3 precursor and KMnO4, the as-obtained MoC/MnO-0.25 CE has superior electrocatalytic ability, low charge transfer resistance and high incident photon-to-current conversion efficiency (IPCE). And the power conversion efficiency of the DSSC based on the MoC/MnO-0.25 CE is up to 8.00%, better than that of the DSSC used standard Pt CE (7.36%) in the same test environment, meanwhile the MoC/MnO-0.25 CE also has good electrochemical stability in the iodine-based electrolyte, which shows a promising candidate to replace Pt for DSSCs.
Vorheriger Artikel Efficient mesoscopic perovskite solar cells from emulsion-based bottom-up self-assembled TiO2 microspheres
Nächster Artikel Alternate lanthanum oxide/silicon oxynitride-based gate stack performance enhancement due to ultrathin oxynitride interfacial layer for CMOS applications

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Metadaten
Titel
MoC/MnO composite materials as high efficient and stable counter electrode catalysts for dye-sensitized solar cells
verfasst von
Aidong Peng
Yuan Gao
Qun Yang
Xueqin Zuo
Huaibao Tang
Guang Li
Publikationsdatum
14.12.2019
Verlag
Springer US
Erschienen in
Journal of Materials Science: Materials in Electronics / Ausgabe 3/2020
Print ISSN: 0957-4522
Elektronische ISSN: 1573-482X
DOI
https://doi.org/10.1007/s10854-019-02717-8

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