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Rheologica Acta

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17.01.2024 | Original Contribution

Rheological behavior of SiO₂ NP/CTAB/PPA wormlike micelles in alcohol/water mixture

verfasst von: Huiying Han, Maen M. Husein, Giovanniantonio Natale

Erschienen in: Rheologica Acta | Ausgabe 2/2024

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Abstract

This study explores the effect of alcohol on the rheological behavior of SiO₂ nanoparticle (NP) in cetyltrimethylammonium bromide (CTAB)/potassium hydrogen phthalate (PPA) wormlike micelles (WLMs). No previous literature explored the effect of chemical stresses on NP-mediated WLMs. The addition of 0.05 wt% NPs increased the zero-shear viscosity of 30 mM CTAB/20 mM PPA WLMs by 30%. A further increase in SiO₂ NPs disrupted the micellar structure, resulting in reduced viscosity. The optimum SiO₂ NP content increased from ~ 0.05 wt% to ~ 0.4 wt% as the CTAB and PPA concentrations increased from 30 mM CTAB/20 mM PPA to 90 mM CTAB/60 mM PPA. The effect of ethanol and 1-hexanol on WLMs composed of 0.05 wt% SiO₂ NP/30 mM CTAB/20 mM PPA was assessed. The NPs enhanced the shear viscosity of ethanol/WLM systems. Notably, at ethanol concentrations of 0.14 wt%, 0.60 wt% and 1.40 wt%, the zero-shear viscosity increased by approximately 60%, 100%, and 25%, respectively. SiO₂ NPs acted as junction points, facilitating the crosslinking among shorter micelles and improving micellar entanglement. Conversely, SiO₂ NPs had little impact on 1-hexanol/WLM systems owing to the strong interaction between WLMs and 1-hexanol at the micellar interface.

Vorheriger Artikel Can numerical methods compete with analytical solutions of linear constitutive models for large amplitude oscillatory shear flow?

Nächster Artikel Rheology and dissolution capacity of cellulose in novel [mTBNH][OAc] ionic liquid mixed with green co-solvents

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Titel: Rheological behavior of SiO2 NP/CTAB/PPA wormlike micelles in alcohol/water mixture
verfasst von: Huiying Han
Maen M. Husein
Giovanniantonio Natale
Publikationsdatum: 17.01.2024
Verlag: Springer Berlin Heidelberg
Erschienen in: Rheologica Acta / Ausgabe 2/2024
Print ISSN: 0035-4511
Elektronische ISSN: 1435-1528
DOI: https://doi.org/10.1007/s00397-024-01432-4

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