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Clean Technologies and Environmental Policy

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30.11.2016 | Original Paper

Catalytic peroxidation of recalcitrant quinoline by ceria impregnated granular activated carbon

verfasst von: Bhawna Yadav, Vimal Chandra Srivastava

Erschienen in: Clean Technologies and Environmental Policy | Ausgabe 5/2017

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Abstract

In this work, quinoline (a recalcitrant poly-nuclear aromatic compound) mineralization was studied by catalytic peroxidation process using ceria impregnated granular activated carbon. Various catalysts with different loading of ceria were prepared by wetness impregnation method and further characterized by liquid nitrogen adsorption–desorption technique, X-ray diffraction, scanning electron microscopy, thermo-gravimetric analysis and Fourier transform infrared spectroscopy. Effects of various parameters like ceria loading, pH, catalyst dose (C _w), H₂O₂/quinoline molar ratio, initial concentration (C _o) of quinoline, reaction temperature (T) and time on quinoline degradation and chemical oxygen demand (COD) removal efficiencies were studied. Quinoline degradation of 81.6% and COD removal of 86.5% were observed at optimum operating condition of pH = 4, C _o = 100 mg/L, Ce loading = 7.5 wt%, H₂O₂/quinoline molar ratio = 1, C _w = 0.5 g/L, T = 55 °C and reaction time = 4 h. The kinetics of the oxidation process was represented by the power law model.

Vorheriger Artikel Bridging LCA data gaps by use of process simulation for energy generation

Nächster Artikel The study of photoelectrochemical properties of LaMnO3, LaFeO3, LaCrO3, and LaNiO3 photoelectrodes for hydrogen production

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Titel: Catalytic peroxidation of recalcitrant quinoline by ceria impregnated granular activated carbon
verfasst von: Bhawna Yadav
Vimal Chandra Srivastava
Publikationsdatum: 30.11.2016
Verlag: Springer Berlin Heidelberg
Erschienen in: Clean Technologies and Environmental Policy / Ausgabe 5/2017
Print ISSN: 1618-954X
Elektronische ISSN: 1618-9558
DOI: https://doi.org/10.1007/s10098-016-1315-8

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