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Environmental Earth Sciences

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01.12.2013 | Special Issue

(Cr_1−xAl_x)N as a candidate for corrosion protection in high temperature segments of CCS plants

verfasst von: W. Garkas, S. Weiß, Q. M. Wang

Erschienen in: Environmental Earth Sciences | Ausgabe 8/2013

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Abstract

Three (Cr_1−xAl_x)N (x = 0.33, 0.5, 0.66) coatings were deposited on Ni-super alloy IN718 using reactive magnetron sputtering. The oxidation behavior of all coatings at 900 °C up to 500 h in air was studied. Furthermore, the corrosion behavior of the (Cr_0.33,Al_0.66)N coating at 900 °C (corrosion type I) by spraying a uniform salt scale of Na₂SO₄ on the sample surface (1 mg/cm²) was investigated. It was found that the coated samples indicate significantly higher oxidation and corrosion resistance compared to uncoated Ni super alloy. This is mainly due to the formation of protective Cr₂O₃ and Al₂O₃ layers on the coating surface. With the increase of Al content, the coatings exhibited improved oxidation resistance. The formation of thin and adherent Al₂O₃ scale on the surface of Al rich coating is the reason for its better oxidation behavior. The detailed structures of the oxide scales and the interdiffusion between coating and substrate were studied using energy dispersive X-ray spectroscopy-analysis.

Vorheriger Artikel CFD modeling of high-pressurized CO2 released from onshore pipeline leakages

Nächster Artikel Sabatier-based CO2-methanation by catalytic conversion

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Titel: (Cr1−x Al x )N as a candidate for corrosion protection in high temperature segments of CCS plants
verfasst von: W. Garkas
S. Weiß
Q. M. Wang
Publikationsdatum: 01.12.2013
Verlag: Springer Berlin Heidelberg
Erschienen in: Environmental Earth Sciences / Ausgabe 8/2013
Print ISSN: 1866-6280
Elektronische ISSN: 1866-6299
DOI: https://doi.org/10.1007/s12665-013-2646-y

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