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Journal of Electronic Materials
Erschienen in: Journal of Electronic Materials 5/2024

02.03.2024 | Original Research Article

Upconversion Spectral Modulation and Temperature Sensing of NaYF4:Yb3+/Ho3+/Tm3+/Gd3+ Nanorods with Resistance to Thermal Quenching

verfasst von: Wei Zhou, Jian Yang, Xiangliang Jin

Erschienen in: Journal of Electronic Materials | Ausgabe 5/2024

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Abstract

Upconversion (UC) nanomaterials are of interest to researchers because of their excellent photostability, effective quantum efficiency and optical temperature dependence. However, most UC nanomaterials are thermally quenched, which causes optical nanothermometers to be susceptible to their own thermal effects, reducing the accuracy of temperature measurements. In this paper, NaYF4:Yb3+/Ho3+/Tm3+/Gd3+ nanorods with UC luminescence and resistance to thermal quenching are prepared through a simple hydrothermal method. The UC luminescence intensity of NaYF4:Yb3+/Ho3+/Tm3+/Gd3+ nanorods is adjusted by doping with Tm3+ ions. The luminescence intensity at each location shows different temperature dependence as the temperature increases. When the temperature reaches 573 K, the integrated luminescence intensity is three times that at 293 K. At the same time, the intensity at all temperature points in the range of 293–573 K is greater than the intensity at 293 K, which shows that the nanorods have excellent resistance to thermal quenching. In addition, the relative sensitivity (Sr) of LIR(I696/I476), LIR(I696/I541), LIR(I696/I646), LIR(I696/I802), and LIR(I541/I476) is investigated based on the luminescence intensity ratio (LIR) technique. The Sr of LIR(I696/I802) is found to have larger values in the low-temperature range, while Sr of LIR(I696/I476) has larger values in the high-temperature range. The use of LIR(I696/I802) and LIR(I696/I476) in separate temperature bands allows Sr to reach 0.93–1.67 %K−1 in the range of 293–573 K, confirming that the nanorods have high Sr over a wide temperature interval. This study indicates that the NaYF4:Yb3+/Ho3+/Tm3+/Gd3+ nanorods are promising candidates for optical thermometers with high sensitivity, wide temperature range, and resistance to thermal quenching.
Vorheriger Artikel Role of Bismuth Doping on Structural and Electrical Properties of ZnO Nanocrystals Prepared by Sol–Gel Method
Nächster Artikel Anti-freezing Dough for Renewable and Reconfigurable Flexible Strain Sensors

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Metadaten
Titel
Upconversion Spectral Modulation and Temperature Sensing of NaYF4:Yb3+/Ho3+/Tm3+/Gd3+ Nanorods with Resistance to Thermal Quenching
verfasst von
Wei Zhou
Jian Yang
Xiangliang Jin
Publikationsdatum
02.03.2024
Verlag
Springer US
Erschienen in
Journal of Electronic Materials / Ausgabe 5/2024
Print ISSN: 0361-5235
Elektronische ISSN: 1543-186X
DOI
https://doi.org/10.1007/s11664-024-10957-6

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