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30.07.2020 | Original Article

Facile fabrication of nanoscale hierarchical porous zeolitic imidazolate frameworks for enhanced toluene adsorption capacity

verfasst von: Min-Hui Yang, Chong-Xiong Duan, Xin-Juan Zeng, Jing-Jing Li, Cui-Yin Liu, Long-Jiao Zeng, Yi Zhang, Kai Wang, Hong-Xia Xi

Erschienen in: Rare Metals | Ausgabe 2/2021

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Abstract

The development of a simple and facile synthesis route is a highly desirable but challenging process in the fabrication of nanoscale hierarchical porous zeolitic imidazolate frameworks (ZIFs). Herein we describe a facile method for rapidly synthesizing hierarchically porous ZIF-90 nanocrystals (particle sizes of ~ 300 nm) using hydroxyl double salts as intermediates at room temperature. The as-synthesized ZIF-90 contained hierarchical porous structures developed using a crystalline interior and a random stack of multiple nanoparticles. Both the morphology and particle size of ZIF-90 nanocrystals could be tuned by controlling the molar ratio of ICA/Zn²⁺. Note that the as-synthesized hierarchically porous ZIF-90 nanocrystals exhibited higher thermal stability compared with the conventional ZIF-90. Because of the introduction of hierarchical porous structures, the resultant hierarchically porous ZIF-90 nanocrystals showed enhanced toluene adsorption capacity than those of conventional metal organic frameworks and zeolites.

Graphic abstract

Vorheriger Artikel Recent advances and perspective in metal coordination materials-based electrode materials for potassium-ion batteries

Nächster Artikel Metal organic framework (ZIF-67)-derived Co nanoparticles/N-doped carbon nanotubes composites for electrochemical detecting of tert-butyl hydroquinone

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Titel: Facile fabrication of nanoscale hierarchical porous zeolitic imidazolate frameworks for enhanced toluene adsorption capacity
verfasst von: Min-Hui Yang
Chong-Xiong Duan
Xin-Juan Zeng
Jing-Jing Li
Cui-Yin Liu
Long-Jiao Zeng
Yi Zhang
Kai Wang
Hong-Xia Xi
Publikationsdatum: 30.07.2020
Verlag: Nonferrous Metals Society of China
Erschienen in: Rare Metals / Ausgabe 2/2021
Print ISSN: 1001-0521
Elektronische ISSN: 1867-7185
DOI: https://doi.org/10.1007/s12598-020-01455-9

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Abstract

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