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Erschienen in: Journal of Materials Engineering and Performance 12/2022

24.05.2022 | Technical Article

Hydrothermal Sealing of Plasma Electrolytic Oxidation Coatings Developed on AZ31 Alloy

Erschienen in: Journal of Materials Engineering and Performance | Ausgabe 12/2022

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Abstract

In this work, a PEO coating on AZ31 magnesium alloy was post-treated in three different solutions containing NaF, Na2CO3 and NaAlO2, with the aim of sealing the anodic film and consequently increasing the corrosion resistance of the material. The morphology and chemical composition of the resulting coatings were analyzed by scanning electron microscopy, x-ray diffraction and Fourier transform infrared spectroscopy. Samples were tested in a salt spray chamber, and corrosion rate was evaluated by the hydrogen evolution technique. It was found that a pore sealing treatment of 90 minutes in the solution containing a mixture of NaF and NaAlO2 resulted in an increase in the corrosion resistance of the PEO coating.

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Literatur
1.
Zurück zum Zitat M.E.E. Alam, S. Han, A.S. Hamouda, Q.B. Nguyen and M. Gupta, Development and Characterization of New AZ41 and AZ51 Magnesium Alloys, Magnesium Technology 2011. W. Sillekens, S. Agnew, N. Neelameggham, S. Mathaudhu Ed., Springer, Cham, 2011, p 553–558 M.E.E. Alam, S. Han, A.S. Hamouda, Q.B. Nguyen and M. Gupta, Development and Characterization of New AZ41 and AZ51 Magnesium Alloys, Magnesium Technology 2011. W. Sillekens, S. Agnew, N. Neelameggham, S. Mathaudhu Ed., Springer, Cham, 2011, p 553–558
14.
Zurück zum Zitat M. Mohedano, P. Pérez, E. Matykina, B. Pillado, G. Garcés and R. Arrabal, PEO Coating with Ce-Sealing for Corrosion Protection of LPSO Mg–Y–Zn Alloy, Surf. Coatings Technol., 2020, 383, p 125253. CrossRef M. Mohedano, P. Pérez, E. Matykina, B. Pillado, G. Garcés and R. Arrabal, PEO Coating with Ce-Sealing for Corrosion Protection of LPSO Mg–Y–Zn Alloy, Surf. Coatings Technol., 2020, 383, p 125253. CrossRef
17.
Zurück zum Zitat A.C. Bouali, E.A. Straumal, M. Serdechnova, D.C.F. Wieland, M. Starykevich, C. Blawert, J.U. Hammel, S.A. Lermontov, M.G.S. Ferreira and M.L. Zheludkevich, Layered Double Hydroxide Based Active Corrosion Protective Sealing of Plasma Electrolytic Oxidation/Sol-Gel Composite Coating on AA2024, Appl. Surf. Sci., 2019, 494, p 829–840. https://doi.org/10.1016/j.apsusc.2019.07.117CrossRef A.C. Bouali, E.A. Straumal, M. Serdechnova, D.C.F. Wieland, M. Starykevich, C. Blawert, J.U. Hammel, S.A. Lermontov, M.G.S. Ferreira and M.L. Zheludkevich, Layered Double Hydroxide Based Active Corrosion Protective Sealing of Plasma Electrolytic Oxidation/Sol-Gel Composite Coating on AA2024, Appl. Surf. Sci., 2019, 494, p 829–840. https://​doi.​org/​10.​1016/​j.​apsusc.​2019.​07.​117CrossRef
24.
Zurück zum Zitat W. Zhang, B. Tian, K.-Q. Du, H.-X. Zhang and F.-H. Wang, Preparation and Corrosion Performance of PEO Coating with Low Porosity on Magnesium Alloy AZ91D in Acidic KF System, Int. J. Electrochem. Sci, 2011, 6, p 5228–5248. W. Zhang, B. Tian, K.-Q. Du, H.-X. Zhang and F.-H. Wang, Preparation and Corrosion Performance of PEO Coating with Low Porosity on Magnesium Alloy AZ91D in Acidic KF System, Int. J. Electrochem. Sci, 2011, 6, p 5228–5248.
25.
Zurück zum Zitat Z. Jiang, X. Zeng and Z. Yao, Preparation of Micro-Arc Oxidation Coatings on Magnesium Alloy and Its Thermal Shock Resistance Property, Rare Met., 2006, 25(3), p 270–273. CrossRef Z. Jiang, X. Zeng and Z. Yao, Preparation of Micro-Arc Oxidation Coatings on Magnesium Alloy and Its Thermal Shock Resistance Property, Rare Met., 2006, 25(3), p 270–273. CrossRef
27.
Zurück zum Zitat G.-H. Lv, H. Chen, X.-Q. Wang, H. Pang, G.-L. Zhang, B. Zou, H.-J. Lee and S.-Z. Yang, Effect of Additives on Structure and Corrosion Resistance of Plasma Electrolytic Oxidation Coatings on AZ91D Magnesium Alloy in Phosphate Based Electrolyte, Surf. Coat. Technol., 2010, 205, p S36–S40. CrossRef G.-H. Lv, H. Chen, X.-Q. Wang, H. Pang, G.-L. Zhang, B. Zou, H.-J. Lee and S.-Z. Yang, Effect of Additives on Structure and Corrosion Resistance of Plasma Electrolytic Oxidation Coatings on AZ91D Magnesium Alloy in Phosphate Based Electrolyte, Surf. Coat. Technol., 2010, 205, p S36–S40. CrossRef
29.
Zurück zum Zitat C. Singh, S.K. Tiwari and R. Singh, Effect of Carbonate and Phosphate Conversion Pretreatments and Optimization on Corrosion Behaviour of Subsequent Electroless Nickel Coating on AZ91 Alloy, Appl. Surf. Sci., 2019, 483, p 334–354. CrossRef C. Singh, S.K. Tiwari and R. Singh, Effect of Carbonate and Phosphate Conversion Pretreatments and Optimization on Corrosion Behaviour of Subsequent Electroless Nickel Coating on AZ91 Alloy, Appl. Surf. Sci., 2019, 483, p 334–354. CrossRef
30.
Zurück zum Zitat L. Toro, A.A. Zuleta, E. Correa, D. Calderón, Y. Galindez, J. Calderón, P. Chacón, A. Valencia-Escobar and F.E. Echeverría, New Insights on the Influence of Low Frequency Pulsed Current on the Characteristics of PEO Coatings Formed on AZ31B, Mater. Res. Express., 2020, 7(1), p 016539. https://doi.org/10.1088/2053-1591/ab61acCrossRef L. Toro, A.A. Zuleta, E. Correa, D. Calderón, Y. Galindez, J. Calderón, P. Chacón, A. Valencia-Escobar and F.E. Echeverría, New Insights on the Influence of Low Frequency Pulsed Current on the Characteristics of PEO Coatings Formed on AZ31B, Mater. Res. Express., 2020, 7(1), p 016539. https://​doi.​org/​10.​1088/​2053-1591/​ab61acCrossRef
31.
Zurück zum Zitat W.S. Rasband and U.S. National Institutes of Health. ImageJ “Bethesda, Maryland, USA, U.S. National Institutes of Health, (2018). W.S. Rasband and U.S. National Institutes of Health. ImageJ “Bethesda, Maryland, USA, U.S. National Institutes of Health, (2018).
32.
Zurück zum Zitat B. Lou, Y. Lin, C. Tseng, Y. Lu, J. Duh and J. Lee, Plasma Electrolytic Oxidation Coatings on AZ31 Magnesium Alloys with Si3N4 Nanoparticle Additives, Surf. Coat. Technol., 2017, 332, p 358–367. CrossRef B. Lou, Y. Lin, C. Tseng, Y. Lu, J. Duh and J. Lee, Plasma Electrolytic Oxidation Coatings on AZ31 Magnesium Alloys with Si3N4 Nanoparticle Additives, Surf. Coat. Technol., 2017, 332, p 358–367. CrossRef
34.
Zurück zum Zitat G. Song, A. Atrens and D. StJohn, An Hydrogen Evolution Method for the Estimation of the Corrosion Rate of Magnesium Alloys, Essential Readings in Magnesium Technology. S.N. Mathaudhu, A.A. Luo, N.R. Neelameggham, E.A. Nyberg, W.H. Sillekens Ed., Springer, Cham, 2016, p 565–572. https://doi.org/10.1007/978-3-319-48099-2_90CrossRef G. Song, A. Atrens and D. StJohn, An Hydrogen Evolution Method for the Estimation of the Corrosion Rate of Magnesium Alloys, Essential Readings in Magnesium Technology. S.N. Mathaudhu, A.A. Luo, N.R. Neelameggham, E.A. Nyberg, W.H. Sillekens Ed., Springer, Cham, 2016, p 565–572. https://​doi.​org/​10.​1007/​978-3-319-48099-2_​90CrossRef
36.
Zurück zum Zitat ASTM B117-18, “Standard Practice for Operating Salt Spray (FOG) Apparatus,” (West Conshohocken, PA), ASTM International, 2018, p 1–15a ASTM B117-18, “Standard Practice for Operating Salt Spray (FOG) Apparatus,” (West Conshohocken, PA), ASTM International, 2018, p 1–15a
37.
Zurück zum Zitat ASTM D610-08, “Standard Test Method for Evaluating Degree of Rusting on Painted Steel Surfaces,” (West Conshohocken, PA), ASTM International, 2008, p 1–6 ASTM D610-08, “Standard Test Method for Evaluating Degree of Rusting on Painted Steel Surfaces,” (West Conshohocken, PA), ASTM International, 2008, p 1–6
38.
Zurück zum Zitat L. Wu, D. Yang, G. Zhang, Z. Zhang, S. Zhang, A. Tang and F. Pan, Fabrication and Characterization of Mg-M Layered Double Hydroxide Films on Anodized Magnesium Alloy AZ31, Appl. Surf. Sci., 2018, 431, p 177–186. CrossRef L. Wu, D. Yang, G. Zhang, Z. Zhang, S. Zhang, A. Tang and F. Pan, Fabrication and Characterization of Mg-M Layered Double Hydroxide Films on Anodized Magnesium Alloy AZ31, Appl. Surf. Sci., 2018, 431, p 177–186. CrossRef
40.
Zurück zum Zitat A. Bautista, J. González and V. López, Influence of Triethanolamine Additions on the Sealing Mechanism of Anodised Aluminium, Surf. Coat. Technol., 2002, 154(1), p 49–54. CrossRef A. Bautista, J. González and V. López, Influence of Triethanolamine Additions on the Sealing Mechanism of Anodised Aluminium, Surf. Coat. Technol., 2002, 154(1), p 49–54. CrossRef
45.
Zurück zum Zitat M. Daroonparvar, M.A.M. Yajid, R.K. Gupta, N.M. Yusof, H.R. Bakhsheshi-Rad and H. Ghandvar, Investigation of Corrosion Protection Performance of Multiphase PEO (Mg2SiO4, MgO, MgAl2O4) Coatings on Mg Alloy Formed in Aluminate-Silicate- Based Mixture Electrolyte, Prot. Met. Phys. Chem. Surfaces, 2018, 54(3), p 425–441. CrossRef M. Daroonparvar, M.A.M. Yajid, R.K. Gupta, N.M. Yusof, H.R. Bakhsheshi-Rad and H. Ghandvar, Investigation of Corrosion Protection Performance of Multiphase PEO (Mg2SiO4, MgO, MgAl2O4) Coatings on Mg Alloy Formed in Aluminate-Silicate- Based Mixture Electrolyte, Prot. Met. Phys. Chem. Surfaces, 2018, 54(3), p 425–441. CrossRef
48.
Zurück zum Zitat J. Dou, Y. Zhao, L. Lu, G. Gu, H. Yu and C. Chen, Effect of the Second-Step Voltages on the Structural and Corrosion Properties of Silicon–Calcium–Phosphate (Si–CaP) Coatings on Mg–Zn–Ca Alloy, R. Soc. Open Sci., 2018, 5(10), p 172410. https://doi.org/10.1098/rsos.172410CrossRef J. Dou, Y. Zhao, L. Lu, G. Gu, H. Yu and C. Chen, Effect of the Second-Step Voltages on the Structural and Corrosion Properties of Silicon–Calcium–Phosphate (Si–CaP) Coatings on Mg–Zn–Ca Alloy, R. Soc. Open Sci., 2018, 5(10), p 172410. https://​doi.​org/​10.​1098/​rsos.​172410CrossRef
51.
Zurück zum Zitat M. Rahmati, K. Raeissi, M.R. Toroghinejad, A. Hakimizad and M. Santamaria, Effect of Pulse Current Mode on Microstructure, Composition and Corrosion Performance of the Coatings Produced by Plasma Electrolytic Oxidation on AZ31 Mg Alloy, Coatings., 2019, 9(10), p 688. CrossRef M. Rahmati, K. Raeissi, M.R. Toroghinejad, A. Hakimizad and M. Santamaria, Effect of Pulse Current Mode on Microstructure, Composition and Corrosion Performance of the Coatings Produced by Plasma Electrolytic Oxidation on AZ31 Mg Alloy, Coatings., 2019, 9(10), p 688. CrossRef
52.
Zurück zum Zitat J. Liang, B. Guo, J. Tian, H. Liu, J. Zhou, W. Liu and T. Xu, Effects of NaAlO2 on Structure and Corrosion Resistance of Microarc Oxidation Coatings Formed on AM60B Magnesium Alloy in Phosphate–KOH Electrolyte, Surf. Coat. Technol., 2005, 199(2–3), p 121–126. CrossRef J. Liang, B. Guo, J. Tian, H. Liu, J. Zhou, W. Liu and T. Xu, Effects of NaAlO2 on Structure and Corrosion Resistance of Microarc Oxidation Coatings Formed on AM60B Magnesium Alloy in Phosphate–KOH Electrolyte, Surf. Coat. Technol., 2005, 199(2–3), p 121–126. CrossRef
54.
Zurück zum Zitat M. Carboneras, L.S. Hernández, J.A. del Valle, M.C. García-Alonso and M.L. Escudero, Corrosion Protection of Different Environmentally Friendly Coatings on Powder Metallurgy Magnesium, J. Alloys Compd., 2010, 496(1–2), p 442–448. CrossRef M. Carboneras, L.S. Hernández, J.A. del Valle, M.C. García-Alonso and M.L. Escudero, Corrosion Protection of Different Environmentally Friendly Coatings on Powder Metallurgy Magnesium, J. Alloys Compd., 2010, 496(1–2), p 442–448. CrossRef
55.
Zurück zum Zitat L. Châtelet, J.Y. Bottero, J. Yvon and A. Bouchelaghem, Competition between Monovalent and Divalent Anions for Calcined and Uncalcined Hydrotalcite: Anion Exchange and Adsorption Sites, Colloids Surf. A Physicochem. Eng. Asp., 1996, 111(3), p 167–175. CrossRef L. Châtelet, J.Y. Bottero, J. Yvon and A. Bouchelaghem, Competition between Monovalent and Divalent Anions for Calcined and Uncalcined Hydrotalcite: Anion Exchange and Adsorption Sites, Colloids Surf. A Physicochem. Eng. Asp., 1996, 111(3), p 167–175. CrossRef
56.
Zurück zum Zitat J. Chen, Y. Song, D. Shan and E. Han, Study of the Corrosion Mechanism of the in Situ Grown Mg–Al–CO32− Hydrotalcite Film on AZ31 Alloy, Corros. Sci., 2012, 65, p 268–277. CrossRef J. Chen, Y. Song, D. Shan and E. Han, Study of the Corrosion Mechanism of the in Situ Grown Mg–Al–CO32− Hydrotalcite Film on AZ31 Alloy, Corros. Sci., 2012, 65, p 268–277. CrossRef
57.
Zurück zum Zitat R C. Ropp, Chapter 5 - Group 14 Alkaline Earth Compounds, RCBT-E of the A.E.C. Ropp, Ed. (Elsevier, Amsterdam, 2013) p 351–480 R C. Ropp, Chapter 5 - Group 14 Alkaline Earth Compounds, RCBT-E of the A.E.C. Ropp, Ed. (Elsevier, Amsterdam, 2013) p 351–480
Metadaten
Titel
Hydrothermal Sealing of Plasma Electrolytic Oxidation Coatings Developed on AZ31 Alloy
Publikationsdatum
24.05.2022
Erschienen in
Journal of Materials Engineering and Performance / Ausgabe 12/2022
Print ISSN: 1059-9495
Elektronische ISSN: 1544-1024
DOI
https://doi.org/10.1007/s11665-022-07028-4

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